含石墨烯(GDY)和其他金属材料的复合材料体系的精确构建促进了创新结构的形成和在能源领域的实际应用,催化作用,光电子学,和生物医学。为了满足实际要求,在宽范围内精确形成多尺度界面,从单原子到纳米结构,在结构设计和性能优化中起着重要作用。结构之间的内在相关性,合成过程,特征属性,并对器件性能进行了系统的研究。本文概述了有关GDY上多尺度金属界面受控形成的最新研究成果。界面调节的综合策略,以及结构和性能之间的相关性,被呈现。此外,还提供了设计和合成负载到GDY基物质上的功能金属基材料的创新研究思路,展示了GDY基材料的应用潜力。
The accurate construction of composite material systems containing
graphdiyne (GDY) and other metallic materials has promoted the formation of innovative structures and practical applications in the fields of energy, catalysis, optoelectronics, and biomedicine. To fulfill the practical requirements, the precise formation of multiscale interfaces over a wide range, from single atoms to nanostructures, plays an important role in the optimization of the structural design and properties. The intrinsic correlations between the structure, synthesis process, characteristic properties, and device performance are systematically investigated. This review outlines the current research achievements regarding the controlled formation of multiscale metallic interfaces on GDY. Synthetic strategies for interface regulation, as well as the correlation between the structure and performance, are presented. Furthermore, innovative research ideas for the design and synthesis of functional metal-based materials loaded onto GDY-based substances are also provided, demonstrating the promising application potential of GDY-based materials.