air quality

空气质量
  • 文章类型: Journal Article
    Retiring coal power plants can reduce air pollution and health damages. However, the spatial distribution of those impacts remains unclear due to complex power system operations and pollution chemistry and transport. Focusing on coal retirements in Pennsylvania (PA), we analyze six counterfactual scenarios for 2019 that differ in retirement targets (e.g., reducing 50% of coal-based installed capacity vs generation) and priorities (e.g., closing plants with higher cost, closer to Environmental Justice Areas, or with higher CO2 emissions). Using a power system model of the PJM Interconnection, we find that coal retirements in PA shift power generation across PA and Rest of PJM, leading to scenario-varying changes in the plant-level release of air pollutants. Considering pollution transport and the size of the exposed population, these emissions changes, in turn, give rise to a reduction of 6-136 PM2.5-attributable deaths in PJM across the six scenarios, with most reductions occurring in PA. Among our designed scenarios, those that reduce more coal power generation yield greater aggregate health benefits due to air quality improvements in PA and adjacent downwind regions. In addition, comparing across the six scenarios evaluated in this study, vulnerable populations─in both PA and Rest of PJM─benefit most in scenarios that prioritize plant closures near Environmental Justice Areas in PA. These results demonstrate the importance of considering cross-regional linkages and sociodemographics in designing equitable retirement strategies.
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  • 文章类型: Journal Article
    我们研究了两种具有不同化学机理的广泛使用的化学传输模型(CTM)的性能,以再现中欧的每日8小时平均臭氧(MDA8O3)负荷。我们从ERA-中期再分析中探索了具有气象学边界条件(BC)的基本案例设置,从CAM-Chem中探索了化学BC,以及基于全局模型场的这些BC中的变化影响。我们的结果表明,气象BC的变化强烈影响与观测值的相关性,但仅略微影响模型偏差,而化学BC的变化增加了模型偏差,而相关模式基本保持不变。此外,我们的研究强调,CTM的选择(和化学机制的选择)对MDA8O3水平的影响与BC改变的影响相似甚至更大。总之,我们的研究呼吁多模型策略结合不同的CTM和BC组合,以探索MDA8O3分布的带宽,从而在后记和未来预测的不确定性,类似于气候研究,考虑在相同的人为排放但初始条件略有不同的情况下进行整体模拟。
    在线版本包含补充材料,可在10.1007/s11869-024-01516-3获得。
    We investigate the performance of two widely used chemistry-transport models (CTMs) with different chemical mechanisms in reproducing the ambient maximum daily 8-h average ozone (MDA8 O3) burden over Central Europe. We explore a base case setup with boundary conditions (BC) for meteorology from the ERA-Interim reanalysis and chemical BC from CAM-Chem as well as effects of alterations in these BC based on global model fields. Our results show that changes in meteorological BC strongly affect the correlation with observations but only marginally affect the model biases, while changes in chemical BC increase model biases while correlation patterns remain largely unchanged. Furthermore, our study highlights that CTM choice (and choice of chemical mechanism) has a similar or even larger impact on MDA8 O3 levels as the impact of altered BC. In summary, our study calls for a multi-model strategy combining different CTM and BC combinations to explore the bandwidth of MDA8 O3 distributions and thus uncertainty in hindcasts and future projections, in analogy to climate studies considering ensemble simulations under the same anthropogenic emissions but with slightly different initial conditions.
    UNASSIGNED: The online version contains supplementary material available at 10.1007/s11869-024-01516-3.
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  • 文章类型: Journal Article
    空气质量差越来越与胃肠道疾病有关,表明与人体肠道健康的潜在相关性。然而,由于研究有限,这种关系在很大程度上仍未被探索。这项研究使用了暴露于食用油烟雾(COFs)和宏基因组学的受控小鼠模型,转录组学,和代谢组学来阐明环境胁迫下肠道菌群与宿主代谢之间的相互作用。我们的研究结果表明,短期COF吸入会在3天内引起肺部炎症并导致胃肠道紊乱,阐明了呼吸道暴露与肠功能障碍的连接途径。暴露强度与肠组织完整性的变化显着相关,微生物组成,和代谢功能。延长7天的暴露会破坏肠道微生物群并改变色氨酸代谢,14天后观察到进一步的变化,突出适应性反应。这些结果突出了肠道健康对空气污染物的脆弱性,并提出了吸入污染物可能影响远处器官系统的途径。
    Poor air quality is increasingly linked to gastrointestinal diseases, suggesting a potential correlation with human intestine health. However, this relationship remains largely unexplored due to limited research. This study used a controlled mouse model exposed to cooking oil fumes (COFs) and metagenomics, transcriptomics, and metabolomics to elucidate interactions between intestine microbiota and host metabolism under environmental stress. Our findings reveal that short-term COF inhalation induces pulmonary inflammation within 3 days and leads to gastrointestinal disturbances, elucidating a pathway connecting respiratory exposure to intestinal dysfunction. The exposure intensity significantly correlates with changes in intestinal tissue integrity, microbial composition, and metabolic function. Extended exposure of 7 days disrupts intestine microbiota and alters tryptophan metabolism, with further changes observed after 14 days, highlighting an adaptive response. These results highlight the vulnerability of intestinal health to airborne pollutants and suggest a pathway through which inhaled pollutants may affect distant organ systems.
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  • 文章类型: Journal Article
    在美国,吸烟是导致过早死亡的主要可预防原因。尝试戒烟是戒烟的重要一步。虽然它已经被广泛研究,有关戒烟尝试与附近空气质量问题之间关联的信息有限。因此,我们研究了过去一年戒烟尝试与吸烟的成年德克萨斯人感知到的邻里空气质量问题之间的关联.
    在2018年,进行了基于横截面多阶段面积概率设计的调查,以收集社会人口统计学,行为,以及来自2050名德克萨斯州居民的代表性样本的健康相关信息。目前的研究包括486名在过去12个月内报告吸烟的成人受访者。使用人口加权多变量逻辑回归分析,检查了戒烟尝试与感知的邻里空气质量(通过自我报告的邻里空气质量问题来衡量)之间的关联。
    总的来说,486名受访者中有60.7%试图戒烟。对于那些报告感知到的邻里空气质量问题的人,尝试戒烟的患病率为74.6%。在多变量分析中,尝试戒烟的可能性较高的患者有感知到的邻里空气质量问题(AOR:1.906[1.104-3.289])和已婚或已婚人士(AOR:1.876[1.161-3.033]).男性尝试戒烟的可能性较低(AOR:0.629[0.397-0.995]),并且随着年龄的增长而降低(AOR:0.968[0.951-0.984])。
    发现的社区空气质量问题可以独立预测德克萨斯州戒烟的尝试。为了鼓励居住在空气质量差的社区的个人戒烟,这些社区应该接受量身定制的循证干预措施,以改善社区教育,社会支持,和医疗保健专业人员协助戒烟。
    UNASSIGNED: Cigarette smoking is the major preventable cause of premature deaths in the United States. Attempting to quit smoking is an important step toward smoking cessation. Although it has been studied extensively, limited information on the association between attempts to quit smoking and neighborhood air quality problems is available. Therefore, we examined the association between attempts to quit smoking in the past year and perceived neighborhood air quality problems among adult Texans who smoke.
    UNASSIGNED: In 2018, a cross-sectional multistage area probability design-based survey was administered to collect sociodemographic, behavioral, and health-related information from a representative sample of 2050 Texas residents. The current study included 486 adult respondents who reported smoking within the past 12 months. The association between attempts to quit smoking and perceived neighborhood air quality (measured by self-reported problems with neighborhood air quality) was examined using a population-weighted multivariable logistic regression analysis.
    UNASSIGNED: Overall, 60.7% of the 486 respondents attempted to quit cigarette smoking. The prevalence of attempting to quit was 74.6% for those reporting perceived neighborhood air quality problems. In the multivariable analysis, a higher likelihood of attempting to quit smoking was found among individuals with perceived neighborhood air quality problems (AOR: 1.906 [1.104-3.289]) and those who were married or living as married (AOR: 1.876 [1.161-3.033]). The likelihood of attempts to quit smoking was lower among males (AOR: 0.629 [0.397-0.995]) and decreased with age (AOR: 0.968 [0.951-0.984]).
    UNASSIGNED: The perceived neighborhood air quality problems were found to independently predict attempts to quit cigarette smoking in Texas. To encourage quitting smoking among individuals living in neighborhoods with poor air quality, such neighborhoods should receive tailored and evidence-based interventions to improve community education, social support, and healthcare professionals\' assistance to quit smoking.
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  • 文章类型: Journal Article
    国内燃烧排放对公众健康构成越来越大的风险,尤其是在英国。现有的反应是两极分化的,政府提倡使用低排放的燃料和炉灶,而清洁空气运动人士呼吁全面禁止燃烧。然而,每种方法控制这些排放的能力都是有限的。在美国可以找到另一种选择,其中“燃烧警报”系统要求炉灶和壁炉用户在实际或预计空气质量差的时期避免照明。鉴于这些制度的有效性,本研究首次设计并评估了英国烧伤警报系统的有效性和可接受性,借鉴行为反应性调节的理论视角。在冬季招募了50名参与者在2周内使用该系统。研究结果表明,自愿烧伤警报系统可以阻止用户之间的燃烧。在收到警报的人中,74%减少燃烧频率或燃烧时间较短。总的来说,警报系统阻止了该组至少178小时的燃烧。定性研究结果表明,行为反应的一致性受技术影响,结构,和环境因素,提供有关如何修改英国烧伤警报系统以提高未来合规性一致性的关键见解。总体结论是,可以在英国及其他地区引入燃烧警报,作为减少家庭燃烧排放及其相关公共卫生风险的手段。
    Domestic combustion emissions pose a growing risk to public health, especially in the UK. Existing responses are polarised, with government advocating use of lower emission fuels and stoves while clean air campaigners call for blanket bans on burning. However, each approach is limited in its ability to control these emissions. An alternative can be found in the U.S.A., where \'burn alert\' systems require stove and fireplace users to avoid lighting during periods of actual or projected poor air quality. Given the effectiveness of these regimes, the current study designs and evaluates the effectiveness and acceptability of a burn alert system in the UK for the first time, drawing on the theoretical perspective of behavioural responsive regulation. Fifty participants were recruited to use the system over 2 weeks in winter. The findings illustrate that a voluntary burn alert system can dissuade burning among users. Of those in receipt of an alert, 74% reduced burning frequency or burned for a shorter duration. In total, the alert system prevented at least 178 hours of burning for this group. Qualitative findings show that the consistency of the behavioural response is influenced by technical, structural, and environmental factors, providing key insight into how UK-based burn alert systems could be modified to increase the consistency of compliance in future. The overall conclusion is that burn alerts could be introduced in the UK and beyond, as a means of reducing domestic combustion emissions and their associated public health risks.
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  • 文章类型: Journal Article
    野火的规模正在增加,频率,和严重性。荒地-城市界面和顺风社区的人口暴露于高浓度的细颗粒物(PM2.5)和野火烟雾的其他有害成分的风险增加。我们进行了这项分析,以评估使用野火烟雾的模型预测来创建县级的烟雾暴露措施,以进行公共卫生研究和监测。
    我们评估了四年(2015-2018年)基于网格的北美中尺度(NAM)从美国森林服务局BlueSky建模框架中得出的PM2.5预测以及来自环境保护署空气质量系统(AQS)的监测数据,受保护的视觉环境的机构间监测(改进),西部区域气候中心(WRCC),以及机构间实时烟雾监测(AIRSIS)计划。为了评估模型导出的估计和基于监控的观察之间的关系,我们通过空间评估了斯皮尔曼的相关性(即,县,城市化水平,受重大野火影响的美国西部各州,和气候区域)和时间(即,月份和野火活动期)特征。然后,我们生成了县级烟雾估计值,并检查了烟雾暴露的总天数和个人天数的时空模式。
    在美国的所有县和所有日子里,县级模型和监测得出的PM2.5估计值之间的相关性为0.14(p<0.001)。使用来自临时监测器的数据以及受高野火烟雾影响的地区和天数的相关性更强,尤其是在美国西部。非大都市县县级模型和监测得出的估计之间的相关性,在较高的浓度范围为0.25至0.54(p<0.001)。
    一般来说,公共卫生从业者和健康研究人员需要考虑与进行健康分析的建模数据产品相关的利弊。我们的结果支持使用模型导出的烟雾估计来识别受重烟事件影响的社区,特别是在紧急响应期间和位于野火事件附近的社区。
    UNASSIGNED: Wildfires are increasing in magnitude, frequency, and severity. Populations in the wildland-urban interface and in downwind communities are at increased risk of exposure to elevated concentrations of fine particulate matter (PM2.5) and other harmful components of wildfire smoke. We conducted this analysis to evaluate the use of modeled predictions of wildfire smoke to create county-level measures of smoke exposure for public health research and surveillance.
    UNASSIGNED: We evaluated four years (2015-2018) of grid-based North American Mesoscale (NAM)-derived PM2.5 forecasts from the U.S. Forest Service BlueSky modeling framework with monitoring data from the Environmental Protection Agency Air Quality System (AQS), the Interagency Monitoring of Protected Visual Environments (IMPROVE), the Western Regional Climate Center (WRCC), and the Interagency Real Time Smoke Monitoring (AIRSIS) programs. To assess relationships between model-derived estimates and monitor-based observations, we assessed Spearman\'s correlations by spatial (i.e., county, level of urbanization, states in the western United States impacted by major wildfires, and climate regions) and temporal (i.e., month and wildfire activity periods) characteristics. We then generated county-level smoke estimates and examined spatial and temporal patterns in total and person-days of smoke exposure.
    UNASSIGNED: Across all counties in the coterminous United States and for all days, the correlation between county-level model- and monitor-derived PM2.5 estimates was 0.14 (p < 0.001). Correlations were stronger using data from temporary monitors and for areas and days impacted by high wildfire smoke, especially in the western United States. Correlations between county-level model- and monitor-derived estimates in non-metropolitan counties, and at higher concentrations ranged from 0.25 to 0.54 (p < 0.001).
    UNASSIGNED: In general, public health practitioners and health researchers need to consider the pros and cons associated with modeled data products for conducting health analyses. Our results support the use of model-derived smoke estimates to identify communities impacted by heavy smoke events, especially during emergency response and for communities located near wildfire episodes.
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  • 文章类型: Journal Article
    本研究调查了2016-2022年山东省空气质量的时空动态。空气质量指数(AQI)显示出季节性规律,由于温度反转和供暖排放,冬季的值较高,在有利的分散条件的帮助下,夏季的数值较低。AQI明显改善,从6.44下降到3.90,下降了约39.4%。沿海城市的空气质量优于内陆地区,受工业活动和地理特征的影响。例如,淄博的地理位置限制了污染物的扩散,导致空气质量差。一氧化碳水平保持稳定,虽然O3在夏季由于光化学反应而季节性增加,相关系数表明与温度有很强的正相关(r=0.65)。冬季,与供暖和车辆排放有关的NO2水平升高,与AQI的相关性增加(r=0.78)。PM2.5和PM10浓度在较冷月份较高,由于加热和大气粉尘,显着下降了45%和40%,分别,在研究期间。预测模型预测空气质量持续改善,取决于持续的政策执行和技术进步。这种方法为未来的空气质量管理和改善提供了一个全面的框架。
    This study investigates the spatial and temporal dynamics of air quality in Shandong Province from 2016 to 2022. The Air Quality Index (AQI) showed a seasonal pattern, with higher values in winter due to temperature inversions and heating emissions, and lower values in summer aided by favorable dispersion conditions. The AQI improved significantly, decreasing by approximately 39.4 % from 6.44 to 3.90. Coastal cities exhibited better air quality than inland areas, influenced by industrial activities and geographical features. For instance, Zibo\'s geography restricts pollutant dispersion, resulting in poor air quality. CO levels remained stable, while O3 increased seasonally due to photochemical reactions in summer, with correlation coefficients indicating a strong positive correlation with temperature (r = 0.65). Winter saw elevated NO2 levels linked to heating and vehicular emissions, with an observed increase in correlation with AQI (r = 0.78). PM2.5 and PM10 concentrations were higher in colder months due to heating and atmospheric dust, showing a significant decrease of 45 % and 40 %, respectively, over the study period. Predictive modeling forecasts continued air quality improvements, contingent on sustained policy enforcement and technological advancements. This approach provides a comprehensive framework for future air quality management and improvement.
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  • 文章类型: Journal Article
    中国柴油卡车是NOx和颗粒物(PM)车辆排放的主要贡献者。柴油卡车的增加可能会加剧空气污染并损害人类健康。中国政府最近实施了一系列排放控制技术和措施,以改善空气质量。本文综述了我国近年来柴油车排放控制技术和措施,并介绍了这些控制技术和措施在京津冀及周边地区的综合应用情况。根据重型柴油卡车的中国VI标准,采用了远程在线监测技术,运输结构调整和重污染企业分类控制等控制措施继续支持污染治理作战行动计划。为推进柴油车排放污染控制和监督提供了观点和建议:坚持统筹管控的理念,大力推广系统技术手段在排放监测中的应用,不断促进货物运输结构调整,推广新能源货运汽车。本文旨在加快在中国各地实施控制技术和措施。中国正在努力控制柴油卡车尾气污染。中国愿与世界合作,保护全球生态环境。
    Chinese diesel trucks are the main contributors to NOx and particulate matter (PM) vehicle emissions. An increase in diesel trucks could aggravate air pollution and damage human health. The Chinese government has recently implemented a series of emission control technologies and measures for air quality improvement. This paper summarizes recent control technologies and measures for diesel truck emissions in China and introduces the comprehensive application of control technologies and measures in Beijing-Tianjin-Hebei and surrounding regions. Remote online monitoring technology has been adopted according to the China VI standard for heavy-duty diesel trucks, and control measures such as transportation structure adjustment and heavy pollution enterprise classification control continue to support the battle action plan for pollution control. Perspectives and suggestions are provided for promoting pollution control and supervision of diesel truck emissions: adhere to the concept of overall management and control, vigorously promote the application of systematic and technological means in emission monitoring, continuously facilitate cargo transportation structure adjustment and promote new energy freight vehicles. This paper aims to accelerate the implementation of control technologies and measures throughout China. China is endeavouring to control diesel truck exhaust pollution. China is willing to cooperate with the world to protect the global ecological environment.
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  • 文章类型: Journal Article
    颗粒硝酸盐(pNO3-)的光解已被认为是对流层中亚硝酸(HONO)的重要来源。然而,确定pNO3-(jpNO3-)的光解速率常数具有很高的不确定性。先前使用气溶胶过滤器对jpNO3进行的实验室测量由于“阴影效应”而变得复杂,“阴影效应”是气溶胶层中的一种消光现象,可能会使这些测量产生偏差。我们开发了一种方法,可以使用具有相同化学成分但不同气溶胶含量的气溶胶过滤器来校正pNO3-对HONO生产的光解速率常数(jpNO3-→HONO)的阴影效应。我们应用该方法量化了冬季霾期间华北平原(NCP)的jpNO3-→HONO。校正阴影效果后,5°C时的归一化平均jpNO3-→HONO从5.89×10-6s-1增加到1.72×10-5s-1。jpNO3-→HONO随pH值和PM2.5中硝酸盐含量的增加而降低,与硝酸盐浓度无关。开发了jpNO3-→HONO的参数化方法,用于在NCP和类似环境中进行HONO生产的模型模拟。
    The photolysis of particulate nitrate (pNO3-) has been suggested to be an important source of nitrous acid (HONO) in the troposphere. However, determining the photolysis rate constant of pNO3- (jpNO3-) suffers from high uncertainty. Prior laboratory measurements of jpNO3- using aerosol filters have been complicated by the \"shadow effect\"─a phenomenon of light extinction within aerosol layers that potentially skews these measurements. We developed a method to correct the shadow effect on the photolysis rate constant of pNO3- for HONO production (jpNO3- → HONO) using aerosol filters with identical chemical compositions but different aerosol loadings. We applied the method to quantify jpNO3- → HONO over the North China Plain (NCP) during the winter haze period. After correcting for the shadow effect, the normalized average jpNO3- → HONO at 5 °C increased from 5.89 × 10-6 s-1 to 1.72 × 10-5 s-1. The jpNO3- → HONO decreased with increasing pH and nitrate proportions in PM2.5 and had no correlation with nitrate concentrations. A parametrization for jpNO3- → HONO was developed for model simulation of HONO production in NCP and similar environments.
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  • 文章类型: Editorial
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