mobile monitoring

移动监控
  • 文章类型: Journal Article
    与传统的固定地点测量相比,移动监测在时间和空间尺度上提供高分辨率观测。这项研究表明,使用GoogleAirView车辆收集的空气污染数据的高时空分辨率来识别热点并评估都柏林市世卫组织空气质量指南(AQG)的遵守情况。流动监察是在平日进行的,通常为2021年5月6日至2022年5月6日之间的7:00至19:00。一秒的数据汇总到377,1138个路段,和8s滚动中位数被汇总到每小时和每天的水平,以便进一步分析。我们评估了细颗粒物(PM2.5)的时间变化,一氧化氮(NO),二氧化氮(NO2),臭氧(O3)一氧化碳(CO),和超局部水平的二氧化碳(CO2)浓度。NO2(28.4±15.7µg/m3)和PM2.5(7.6±4.7µg/m3)的白天平均中值浓度超过了世卫组织24小时(24小时)空气质量指南的49.4%和9%的1年采样时间,分别。对于测得的污染物的日变化,早晨(8:00)和傍晚(18:00)显示NO2和PM2.5的浓度较高,主要发生在冬季,而下午是除O3以外污染最少的时间。低百分位方法以及1小时和白天的最小值方法允许将污染物时间序列分解为背景和局部贡献。NO2和PM2.5的背景贡献随季节变化而变化。当地对PM2.5的贡献略有变化;然而,NO2显示出与交通排放有关的显着的昼夜和季节性变化。短期事件增强(1分钟至1小时)占NO2和PM2.5总浓度的36.0-40.6%和20.8-42.2%。高污染天数占NO2总量的56.3%,突出表明当地交通是短期NO2浓度的主要原因。寿命较长的事件(>8小时)的增强占监测浓度的25%。此外,进行最佳热点分析可以绘制高污染日PM2.5和NO2“热点”点的空间分布图。总的来说,这项调查表明,背景和当地排放都会导致城市地区的PM2.5和NO2污染,并强调迫切需要减轻都柏林交通污染造成的NO2。
    Mobile monitoring provides high-resolution observation on temporal and spatial scales compared to traditional fixed-site measurement. This study demonstrates the use of high spatio-temporal resolution of air pollution data collected by Google Air View vehicles to identify hotspots and assess compliance with WHO Air Quality Guidelines (AQGs) in Dublin City. The mobile monitoring was conducted during weekdays, typically from 7:00 to 19:00, between 6 May 2021 and 6 May 2022. One-second data were aggregated to 377,113 8 s road segments, and 8 s rolling medians were aggregated to hourly and daily levels for further analysis. We assessed the temporal variability of fine particulate matter (PM2.5), nitrogen monoxide (NO), nitrogen dioxide (NO2), ozone (O3), carbon monoxide (CO), and carbon dioxide (CO2) concentrations at hyperlocal levels. The average daytime median concentrations of NO2 (28.4 ± 15.7 µg/m3) and PM2.5 (7.6 ± 4.7 µg/m3) exceeded the WHO twenty-four hours (24 h) Air Quality Guidelines in 49.4% and 9% of the 1-year sampling time, respectively. For the diurnal variation of measured pollutants, the morning (8:00) and early evening (18:00) showed higher concentrations for NO2 and PM2.5, mostly happening in the winter season, while the afternoon is the least polluted time except for O3. The low-percentile approach along with 1-h and daytime minima method allowed for decomposing pollutant time series into the background and local contributions. Background contributions for NO2 and PM2.5 changed along with the seasonal variation. Local contributions for PM2.5 changed slightly; however, NO2 showed significant diurnal and seasonal variability related to traffic emissions. Short-lived event enhancement (1 min to 1 h) accounts for 36.0-40.6% and 20.8-42.2% of the total concentration for NO2 and PM2.5. The highly polluted days account for 56.3% of total NO2, highlighting local traffic is the dominant contributor to short-term NO2 concentrations. The longer-lived events (> 8 h) enhancement accounts for 25% of the monitored concentrations. Additionally, conducting optimal hotspot analysis enables mapping the spatial distribution of \"hot\" spots for PM2.5 and NO2 on highly polluted days. Overall, this investigation suggests both background and local emissions contribute to PM2.5 and NO2 pollution in urban areas and emphasize the urgent need for mitigating NO2 from traffic pollution in Dublin.
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  • 文章类型: Journal Article
    城市热岛(UHI)被认为会对人类健康产生有害影响,这是现代城市面临的主要人为挑战之一。由于城市动态的复杂性,需要进行全面的小气候解码,以设计量身定制的缓解策略,以减少与热量相关的脆弱性。这项研究首次结合了由固定和移动技术组成的两个专用监测系统,提出了一种评估城市内部小气候变异性的新方法。来自三个固定气象站的数据被用来分析长期趋势,在夏季和冬季进行的短期监测活动中使用移动设备(车辆和可穿戴设备)来评估和定位小气候的空间变化。此外,来自移动设备的数据用作佛罗伦萨(意大利)市区Kriging插值的输入,作为案例研究。移动监测会议提供了高分辨率空间数据,能够检测空气温度的超局部变化。使用可穿戴系统验证了最高气温幅度:夏季中午为3.3°C,冬季早晨为4.3°C。在比较绿色区域及其相邻的建筑区时,生理等效温度(PET)被证明是相似的,展示了绿色植物在其周围的微气候缓解贡献。结果还表明,混合两种数据采集和多种分析技术成功地调查了UHI和潜在缓解行动的特定地点作用。此外,移动数据集通过插值监控参数来制作地图是可靠的。插值结果还证明了通过关注目标街道和一天中的时间来优化移动监控活动的可能性,因为插值误差仅在输入样本减少的情况下增加了10%。这允许更好地检测特定于站点的粒度,这对城市规划和决策很重要,适应,和减轻风险的行动,以克服UHI和人为气候变化的影响。
    Urban Heat Island (UHI) is acknowledged to generate harmful consequences on human health, and it is one of the main anthropogenic challenges to face in modern cities. Due to the urban dynamic complexity, a full microclimate decoding is required to design tailored mitigation strategies for reducing heat-related vulnerability. This study proposes a new method to assess intra-urban microclimate variability by combining for the first time two dedicated monitoring systems consisting of fixed and mobile techniques. Data from three fixed weather stations were used to analyze long-term trends, while mobile devices (a vehicle and a wearable) were used in short-term monitoring campaigns conducted in summer and winter to assess and geo-locate microclimate spatial variations. Additionally, data from mobile devices were used as input for Kriging interpolation in the urban area of Florence (Italy) as case study. Mobile monitoring sessions provided high-resolution spatial data, enabling the detection of hyperlocal variations in air temperature. The maximum air temperature amplitudes were verified with the wearable system: 3.3 °C in summer midday and 4.3 °C in winter morning. Physiological Equivalent Temperature (PET) demonstrated to be similar when comparing green areas and their adjacent built-up zone, showing up the microclimate mitigation contribution of greenery in its surrounding. Results also showed that mixing the two data acquisition and varied analysis techniques succeeded in investigating the UHI and the site-specific role of potential mitigation actions. Moreover, mobile dataset was reliable for elaborating maps by interpolating the monitored parameters. Interpolation results demonstrated the possibility of optimizing mobile monitoring campaigns by focusing on targeted streets and times of day since interpolation errors increased by 10% only with properly reduced and simplified input samples. This allowed an enhanced detection of the site-specific granularity, which is important for urban planning and policymaking, adaptation, and risk mitigation actions to overcome the UHI and anthropogenic climate change effects.
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  • 文章类型: Journal Article
    在暴露评估中忽略室内空气质量可能会导致有偏差的暴露估计和关于暴露对健康的影响和环境健康差异的错误结论。这项研究通过比较100个人的两种类型的个人暴露估计值来评估这些偏差:一种来自使用低成本便携式空气监测仪(GeoAir2.0)在室内和室外收集的实时颗粒物(PM2.5)测量结果,另一种来自PurpleAir传感器网络数据仅在室外收集。PurpleAir测量数据用于使用地统计学方法创建光滑的空气污染表面。为了获得基于移动性的暴露估计,两组空气污染数据与个人GPS跟踪数据相结合。然后进行配对样本t检验以检查这两个估计之间的差异。这项研究还调查了基于GeoAir2.0和PurpleAir的估计是否通过进行Welcht检验和ANOVA并比较其t值和F值,得出了有关性别和经济差异的一致结论。这项研究揭示了基于GeoAir2.0和PurpleAir的估计之间的显著差异,PurpleAir数据始终高估暴露(t=5.94;p<0.001)。研究还发现,女性的平均暴露量高于男性(15.65。8.55μg/m3),根据GeoAir2.0数据(t=4.654;p=0.055),可能是由于在室内花费更多时间参与传统上与女性相关的污染产生活动,比如做饭。这与PurpleAir的数据形成对比,这表明男性的暴露量较高(43.78对比。46.26μg/m3)(t=3.793;p=0.821)。此外,GeoAir2.0数据显示出显著的经济差异(F=7.512;p<0.002),低收入群体经历更高的暴露-PurpleAir数据没有捕捉到的差异(F=0.756;p<0.474)。这些发现强调了同时考虑室内和室外空气质量以减少暴露估计偏差并更准确地表示环境差异的重要性。
    Neglecting indoor air quality in exposure assessments may lead to biased exposure estimates and erroneous conclusions about the health impacts of exposure and environmental health disparities. This study assessed these biases by comparing two types of personal exposure estimates for 100 individuals: one derived from real-time particulate matter (PM2.5) measurements collected both indoors and outdoors using a low-cost portable air monitor (GeoAir2.0) and the other from PurpleAir sensor network data collected exclusively outdoors. The PurpleAir measurement data were used to create smooth air pollution surfaces using geostatistical methods. To obtain mobility-based exposure estimates, both sets of air pollution data were combined with the individuals\' GPS tracking data. Paired-sample t-tests were then performed to examine the differences between these two estimates. This study also investigated whether GeoAir2.0- and PurpleAir-based estimates yielded consistent conclusions about gender and economic disparities in exposure by performing Welch\'s t-tests and ANOVAs and comparing their t-values and F-values. The study revealed significant discrepancies between GeoAir2.0- and PurpleAir-based estimates, with PurpleAir data consistently overestimating exposure (t = 5.94; p < 0.001). It also found that females displayed a higher average exposure than males (15.65 versus. 8.55 μg/m3) according to GeoAir2.0 data (t = 4.654; p = 0.055), potentially due to greater time spent indoors engaging in pollution-generating activities traditionally associated with females, such as cooking. This contrasted with the PurpleAir data, which indicated higher exposure for males (43.78 versus. 46.26 μg/m3) (t = 3.793; p = 0.821). Additionally, GeoAir2.0 data revealed significant economic disparities (F = 7.512; p < 0.002), with lower-income groups experiencing higher exposure-a disparity not captured by PurpleAir data (F = 0.756; p < 0.474). These findings highlight the importance of considering both indoor and outdoor air quality to reduce bias in exposure estimates and more accurately represent environmental disparities.
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  • 文章类型: Journal Article
    在附近的街区,居民更频繁地暴露于交通相关的空气污染(TRAP),他们越来越意识到污染水平。考虑到这一点,这项研究采用便携式空气污染物传感器在两个附近的道路社区进行移动监测活动,一个在城市地区,一个在上海郊区,中国。该活动以细颗粒物(PM2.5)和黑碳(BC)的时空分布为特征,以帮助确定这些近路微环境中的适当缓解措施。该研究确定了更高的平均TRAP浓度(PM2.5和BC分别高4.7倍和1.7倍,分别),较低的空间变异性,与夏季相比,冬季污染物间的相关性更强。还研究了TRAP在高峰时间和非高峰时间之间的时间变化。确定地区级PM2.5增量从非高峰时段到高峰时段发生,BC浓度更多地归因于交通排放。此外,社区内TRAP的时空分布表明,PM2.5浓度呈现巨大的时间变异性,但在空间上几乎保持不变,而BC浓度表现出明显的时空变异性。这些发现为TRAP在不同的近路社区的独特时空分布提供了有价值的见解,强调超本地监测在城市微环境中的重要作用,以支持量身定制的设计和实施适当的缓解措施。
    In near-road neighborhoods, residents are more frequently exposed to traffic-related air pollution (TRAP), and they are increasingly aware of pollution levels. Given this consideration, this study adopted portable air pollutant sensors to conduct a mobile monitoring campaign in two near-road neighborhoods, one in an urban area and one in a suburban area of Shanghai, China. The campaign characterized spatiotemporal distributions of fine particulate matter (PM2.5) and black carbon (BC) to help identify appropriate mitigation measures in these near-road micro-environments. The study identified higher mean TRAP concentrations (up to 4.7-fold and 1.7-fold higher for PM2.5 and BC, respectively), lower spatial variability, and a stronger inter-pollutant correlation in winter compared to summer. The temporal variations of TRAP between peak hour and off-peak hour were also investigated. It was identified that district-level PM2.5 increments occurred from off-peak to peak hours, with BC concentrations attributed more to traffic emissions. In addition, the spatiotemporal distribution of TRAP inside neighborhoods revealed that PM2.5 concentrations presented great temporal variability but almost remained invariant in space, while the BC concentrations showed notable spatiotemporal variability. These findings provide valuable insights into the unique spatiotemporal distributions of TRAP in different near-road neighborhoods, highlighting the important role of hyperlocal monitoring in urban micro-environments to support tailored designing and implementing appropriate mitigation measures.
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  • 文章类型: Journal Article
    城市空气污染可能在空间和时间上变化很大。然而,很少有监测策略可以同时解决精细尺度的时空变化。这里,我们提出了一种新的测量驱动的时空建模方法,该方法超越了两种互补采样范式的局限性:移动监测和固定位置传感器网络。我们发展,验证,并应用该模型使用来自密集的数据来预测黑碳(BC),在西奥克兰进行100天的实地研究,CA.我们的时空模型利用了从多污染物移动监测活动中得出的相干空间模式,以填补来自低成本传感器网络的时间完整的BC数据中的空间空白。我们的模型在精细的空间和时间分辨率(30m,15分钟),证明了移动(Pearson的R〜0.77)和固定站点测量(R〜0.95)的样本外相关性强,同时揭示了单独使用单一监测方法无法有效捕获的特征。该模型揭示了主要排放源附近的急剧浓度梯度,同时捕获了它们的时间变异性,提供对污染源和动态的宝贵见解。
    Urban air pollution can vary sharply in space and time. However, few monitoring strategies can concurrently resolve spatial and temporal variation at fine scales. Here, we present a new measurement-driven spatiotemporal modeling approach that transcends the individual limitations of two complementary sampling paradigms: mobile monitoring and fixed-site sensor networks. We develop, validate, and apply this model to predict black carbon (BC) using data from an intensive, 100-day field study in West Oakland, CA. Our spatiotemporal model exploits coherent spatial patterns derived from a multipollutant mobile monitoring campaign to fill spatial gaps in time-complete BC data from a low-cost sensor network. Our model performs well in reconstructing patterns at fine spatial and temporal resolution (30 m, 15 min), demonstrating strong out-of-sample correlations for both mobile (Pearson\'s R ∼ 0.77) and fixed-site measurements (R ∼ 0.95) while revealing features that are not effectively captured by a single monitoring approach in isolation. The model reveals sharp concentration gradients near major emission sources while capturing their temporal variability, offering valuable insights into pollution sources and dynamics.
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  • 文章类型: Journal Article
    空气污染物的高分辨率空间和时空模型的开发对于暴露科学和流行病学应用至关重要。虽然固定地点抽样通常为统计预测模型提供输入数据,不断发展的移动监测方法提供了改进的空间分辨率,非常适合测量具有高空间变异性的污染物,如超细颗粒(UFP)。魁北克空气污染暴露和流行病学(QAPEE)研究测量并模拟了未研究污染物的时空分布,如UFP,黑碳(BC),和棕色碳(BrC),与细颗粒物(PM2.5)一起,二氧化氮(NO2),和臭氧(O3)在魁北克市,加拿大。我们进行了固定现场(NO2和O3)和移动监测(PM2.5,BC,BRC,和UFP)超过10个月的活动。移动监控路线在上午8点至上午10点之间每周进行监控,并使用位置/分配建模进行设计。季节性固定地点采样活动在两周内连续24小时测量。灵活的广义可加模型(GAMs),结合了污染浓度的数据,空间和时空GIS预测因子,以及空间和时间术语,用于对浓度曲面进行建模和预测。PM2.5,NO2,O3以及UFP范围内七个最小尺寸分数的年度模型,具有较高的样本外预测准确性(r2范围:0.54-0.86)。在以颗粒数量计数(PNC)测量的UFP尺寸范围内观察到不同的空间模式。PM2.5的月度时空模型(r2=0.49),BC(r2=0.27),BrC(r2=0.29),和PNC(r2=0.49)具有中等或中低的样本预测准确性。我们进行了敏感性分析,发现对每年代表性的空气污染浓度进行建模所需的\'n访问\'(移动监控会话)的最小次数在24到32次之间,具体取决于污染物。这项研究为魁北克市的一组全面的空气污染物提供了预测暴露模型的单一来源,加拿大。这些暴露模型将纳入环境UFP和其他污染物对健康影响的流行病学研究。
    The development of high-resolution spatial and spatiotemporal models of air pollutants is essential for exposure science and epidemiological applications. While fixed-site sampling has conventionally provided input data for statistical predictive models, the evolving mobile monitoring method offers improved spatial resolution, ideal for measuring pollutants with high spatial variability such as ultrafine particles (UFP). The Quebec Air Pollution Exposure and Epidemiology (QAPEE) study measured and modelled the spatial and spatiotemporal distributions of understudied pollutants, such as UFPs, black carbon (BC), and brown carbon (BrC), along with fine particulate matter (PM2.5), nitrogen dioxide (NO2), and ozone (O3) in Quebec City, Canada. We conducted a combined fixed-site (NO2 and O3) and mobile monitoring (PM2.5, BC, BrC, and UFPs) campaign over 10-months. Mobile monitoring routes were monitored on a weekly basis between 8am-10am and designed using location/allocation modelling. Seasonal fixed-site sampling campaigns captured continuous 24-h measurements over two-week periods. Generalized Additive Models (GAMs), which combined data on pollution concentrations with spatial, temporal, and spatiotemporal predictor variables were used to model and predict concentration surfaces. Annual models for PM2.5, NO2, O3 as well as seven of the smallest size fractions in the UFP range, had high out of sample predictive accuracy (range r2: 0.54-0.86). Varying spatial patterns were observed across UFP size ranges measured as Particle Number Counts (PNC). The monthly spatiotemporal models for PM2.5 (r2 = 0.49), BC (r2 = 0.27), BrC (r2 = 0.29), and PNC (r2 = 0.49) had moderate or moderate-low out of sample predictive accuracy. We conducted a sensitivity analysis and found that the minimum number of \'n visits\' (mobile monitoring sessions) required to model annually representative air pollution concentrations was between 24 and 32 visits dependent on the pollutant. This study provides a single source of exposure models for a comprehensive set of air pollutants in Quebec City, Canada. These exposure models will feed into epidemiological research on the health impacts of ambient UFPs and other pollutants.
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  • 文章类型: Journal Article
    环氧乙烷(“EtO”)是一种工业化生产的挥发性有机化合物,是一种已知的人类致癌物质。关于生产和最终用途设施周围的环境EtO浓度的可靠报告很少,然而,尽管存在重大风险。我们在原地展示,快速(1Hz),2023年2月在路易斯安那州东南部工业走廊进行了敏感的ETO测量。我们以500m的空间分辨率汇总了移动数据,并报告了走廊75km的平均混合比。平均值和中值合计值分别为31.4和23.3ppt,分别,大多数(75%)500米网格单元高于10.9ppt,终生暴露浓度对应于100万分之一的超额癌症风险(1×10-4)。一小部分(3.3%)高于109个百分点(100万分之一的癌症风险,1×10-3);这些往往靠近EtO排放设施,尽管我们观察到距离最近设施超过10公里的羽流。许多羽流与其他测量气体高度相关,指示潜在的排放源,用第二个商用分析仪同时测量一个子集,表现出良好的协议。我们估计了13个人口普查区的EtO,所有这些都高于EPA的估计值(中位数差异为21.3ppt)。我们的发现提供了有关关键工业地区EtO浓度和潜在暴露风险的重要信息,并促进了EtO分析方法在环境采样和空气毒物移动监测中的应用。
    Ethylene oxide (\"EtO\") is an industrially made volatile organic compound and a known human carcinogen. There are few reliable reports of ambient EtO concentrations around production and end-use facilities, however, despite major exposure concerns. We present in situ, fast (1 Hz), sensitive EtO measurements made during February 2023 across the southeastern Louisiana industrial corridor. We aggregated mobile data at 500 m spatial resolution and reported average mixing ratios for 75 km of the corridor. Mean and median aggregated values were 31.4 and 23.3 ppt, respectively, and a majority (75%) of 500 m grid cells were above 10.9 ppt, the lifetime exposure concentration corresponding to 100-in-one million excess cancer risk (1 × 10-4). A small subset (3.3%) were above 109 ppt (1000-in-one million cancer risk, 1 × 10-3); these tended to be near EtO-emitting facilities, though we observed plumes over 10 km from the nearest facilities. Many plumes were highly correlated with other measured gases, indicating potential emission sources, and a subset was measured simultaneously with a second commercial analyzer, showing good agreement. We estimated EtO for 13 census tracts, all of which were higher than EPA estimates (median difference of 21.3 ppt). Our findings provide important information about EtO concentrations and potential exposure risks in a key industrial region and advance the application of EtO analytical methods for ambient sampling and mobile monitoring for air toxics.
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  • 文章类型: Journal Article
    有智力障碍(ID)的人有患糖尿病(DM)和糖尿病性周围神经病变(DPN)的风险,会导致足部溃疡和下肢截肢。然而,认知差异和沟通障碍可能会阻碍某些筛查和预防DPN的方法。可穿戴和移动技术——如智能手机应用程序和压敏鞋垫——可能有助于抵消这些障碍。然而,对这些技术在有身份证的个体中的有效性知之甚少。
    我们对数据库Embase进行了范围审查,PubMed,和WebofScience使用DM的搜索词,DPN,ID,以及诊断或监测DPN的技术。发现缺乏这方面的研究,我们扩大了搜索范围,包括任何有关诊断或监测DPN技术的文献,然后将这些发现应用于ID.
    我们确定了88篇文章;88篇文章中有43篇(48.9%)与步态力学或脚部压力有关。没有文章明确将有身份证的个人作为目标人群,尽管有三篇文章涉及具有其他认知障碍的个体(有中风史的患者中有两篇,血液透析相关认知改变患者中的1例)。
    在使用技术诊断或监测DPN的研究中不代表具有ID的个人。考虑到ID患者中DM并发症的风险以及此类技术减少筛查和预防障碍的潜在额外益处,这是一个令人担忧的问题。更多的研究应该研究如何在有ID的患者中使用可穿戴设备。
    UNASSIGNED: Individuals with intellectual disabilities (IDs) are at risk of diabetes mellitus (DM) and diabetic peripheral neuropathy (DPN), which can lead to foot ulcers and lower-extremity amputations. However, cognitive differences and communication barriers may impede some methods for screening and prevention of DPN. Wearable and mobile technologies-such as smartphone apps and pressure-sensitive insoles-could help to offset these barriers, yet little is known about the effectiveness of these technologies among individuals with ID.
    UNASSIGNED: We conducted a scoping review of the databases Embase, PubMed, and Web of Science using search terms for DM, DPN, ID, and technology to diagnose or monitor DPN. Finding a lack of research in this area, we broadened our search terms to include any literature on technology to diagnose or monitor DPN and then applied these findings within the context of ID.
    UNASSIGNED: We identified 88 articles; 43 of 88 (48.9%) articles were concerned with gait mechanics or foot pressures. No articles explicitly included individuals with ID as the target population, although three articles involved individuals with other cognitive impairments (two among patients with a history of stroke, one among patients with hemodialysis-related cognitive changes).
    UNASSIGNED: Individuals with ID are not represented in studies using technology to diagnose or monitor DPN. This is a concern given the risk of DM complications among patients with ID and the potential for added benefit of such technologies to reduce barriers to screening and prevention. More studies should investigate how wearable devices can be used among patients with ID.
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  • 文章类型: Journal Article
    移动监测活动有效地捕获了受管制和不受管制的空气污染物的长期平均浓度的空间超局部变化。然而,它们在估计时空变化地图中的应用很少被研究。解决这个差距,我们调查了移动测量是否可以评估一天中每小时的长期平均二氧化氮(NO2)浓度.使用在阿姆斯特丹监测了10个月的移动NO2数据,我们研究了两种时空土地利用回归(LUR)方法的性能,时空克里格法和GTWR(地理和时间加权回归),以及每小时分别开发的两个经典空间LUR模型。我们发现移动测量遵循固定现场测量的一般模式,但有相当大的偏差(表明收集的不确定性)。利用异质时空自相关,GTWR平滑了这些偏差,并实现了R2为0.49的整体性能和6.33μg/m3的平均绝对误差,并通过长期固定现场测量(样本外)进行了验证。测试的其他模型受收集不确定性的影响更大。我们强调,移动测量中捕获的时空变化可用于重建长期平均每小时空气污染图。这些地图有助于考虑时空人类活动模式的动态暴露评估。
    Mobile monitoring campaigns have effectively captured spatial hyperlocal variations in long-term average concentrations of regulated and unregulated air pollutants. However, their application in estimating spatiotemporally varying maps has rarely been investigated. Tackling this gap, we investigated whether mobile measurements can assess long-term average nitrogen dioxide (NO2) concentrations for each hour of the day. Using mobile NO2 data monitored for 10 months in Amsterdam, we examined the performance of two spatiotemporal land use regression (LUR) methods, Spatiotemporal-Kriging and GTWR (Geographical and Temporal Weighted Regression), alongside two classical spatial LUR models developed separately for each hour. We found that mobile measurements follow the general pattern of fixed-site measurements, but with considerable deviations (indicating collection uncertainty). Leveraging heterogeneous spatiotemporal autocorrelations, GTWR smoothed these deviations and achieved an overall performance of an R2 of 0.49 and a Mean Absolute Error of 6.33 μg/m3, validated by long-term fixed-site measurements (out-of-sample). The other models tested were more affected by the collection uncertainty. We highlighted that the spatiotemporal variations captured in mobile measurements can be used to reconstruct long-term average hourly air pollution maps. These maps facilitate dynamic exposure assessments considering spatiotemporal human activity patterns.
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  • 文章类型: Journal Article
    使用低成本传感器(LCS)进行石油和天然气排放的移动监测是低成本空气质量监测设备的一项研究不足的应用。为了评估低成本传感器作为移动监测源自科罗拉多州东部井场的逃逸甲烷排放的筛查工具的有效性,从2023年8月15日至9月27日,我们将一系列低成本传感器(XPOD)与参考级甲烷监测器(AerisUltra)放在移动监测车上。使用引导和聚合随机森林模型拟合我们的低成本传感器数据,我们发现参考和XPODCH4浓度之间的高度相关性(r=0.719)和低实验误差(RMSD=0.3673ppm)。其他校准模型,包括多元线性回归和人工神经网络(ANN),与随机森林模型相比,要么无法区分基线以上的单个甲烷峰值,要么具有显着升高的误差(RMSDANN=0.4669ppm)。使用包外预测器排列,我们发现与甲烷相关性最高的传感器在我们的随机森林模型中显示出最大的意义。随着我们减少随机森林模型中使用的托管数据的百分比,误差没有显著增加,直到特定阈值(总校准数据的50%).使用寻峰算法,我们发现,我们的模型能够预测80%的甲烷峰值超过2.5ppm,错误的回应率为35%。
    The use of low-cost sensors (LCSs) for the mobile monitoring of oil and gas emissions is an understudied application of low-cost air quality monitoring devices. To assess the efficacy of low-cost sensors as a screening tool for the mobile monitoring of fugitive methane emissions stemming from well sites in eastern Colorado, we colocated an array of low-cost sensors (XPOD) with a reference grade methane monitor (Aeris Ultra) on a mobile monitoring vehicle from 15 August through 27 September 2023. Fitting our low-cost sensor data with a bootstrap and aggregated random forest model, we found a high correlation between the reference and XPOD CH4 concentrations (r = 0.719) and a low experimental error (RMSD = 0.3673 ppm). Other calibration models, including multilinear regression and artificial neural networks (ANN), were either unable to distinguish individual methane spikes above baseline or had a significantly elevated error (RMSDANN = 0.4669 ppm) when compared to the random forest model. Using out-of-bag predictor permutations, we found that sensors that showed the highest correlation with methane displayed the greatest significance in our random forest model. As we reduced the percentage of colocation data employed in the random forest model, errors did not significantly increase until a specific threshold (50 percent of total calibration data). Using a peakfinding algorithm, we found that our model was able to predict 80 percent of methane spikes above 2.5 ppm throughout the duration of our field campaign, with a false response rate of 35 percent.
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