137Cs

137Cs
  • 文章类型: Journal Article
    The invasion of Ukraine and military operations around Ukrainian nuclear power plants and other nuclear facilities have prompted us to search for radiocaesium in mosses from the Kopački Rit Nature Park in Croatia, since mosses are known bioindicators of airborne radioactive pollution, and Kopački Rit is a known low radiocaesium background area. Sampling was finished in August 2023, and our analysis found no elevated radiocaesium levels. Kopački Rit therefore remains a suitable place for future detection of anthropogenic radioactive pollutants.
    Invazija na Ukrajinu i vojne operacije oko ukrajinskih nuklearnih elektrana i drugih nuklearnih postrojenja potaknule su nas da potražimo radiocezij u mahovinama u Parku prirode Kopački rit, jer su mahovine poznati bioindikatori radioaktivnog onečišćenja zraka, a Kopački je rit poznat po niskoj razini onečišćenja radiocezijem. Uzorkovanje je završeno u kolovozu 2023. Naša analiza nije otkrila povišene razine radiocezija. Kopački rit stoga ostaje pogodno mjesto za buduću detekciju antropogenog radioaktivnog onečišćenja.
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  • 文章类型: Journal Article
    瑞典成年男性的癌症风险增加与切尔诺贝利事故对结肠的吸收剂量增加有关。
    一个封闭队列,有猎人身份的信息,包括1986年生活在瑞典北部的所有个人。共有2,104,101人获得了有关在住宅坐标处接触137Cs的完整年度信息。一种巢式病例对照方法,四个对照匹配癌症诊断年份和出生年份,被使用。在1986年至2020年之间计算了个体器官吸收剂量,包括外部和内部暴露。使用针对农村/非农村栖息地调整后的条件逻辑回归计算每mGy的危害比(HR)和95%置信区间(95%CI)。1980年至1985年的教育水平和切尔诺贝利前癌症发病率。共纳入男性161,325例癌症病例和女性144,439例癌症病例。
    所有癌症部位合并的每mGy的校正HR在男性中为1.027(95%CI=1.022,1.031),在女性中为1.011(95%CI=1.006,1.017)。在事后分析中,考虑了猎人生活方式和县切尔诺贝利前癌症发病率的混淆,所有合并癌症部位的校正HR/mGy男性为1.014(95%CI=1.009,1.019),女性为1.000(95%CI=0.994,1.006).事后分析表明结肠癌的风险增加,胰腺,和胃,分别,在男性中,女性淋巴瘤。
    发现某些特定癌症部位的癌症风险估计增加,但不能排除由于猎人的生活方式而导致的不受控制的混杂因素。
    UNASSIGNED: Adult males in Sweden exhibit an increased risk of cancer associated with an increased absorbed dose to the colon from the Chernobyl accident.
    UNASSIGNED: A closed cohort, with information on hunter status, included all individuals living in northern Sweden in 1986. Complete annual information on exposure to 137Cs at the dwelling coordinate was available for a total of 2,104,101 individuals. A nested case-control method with four controls matched for year of cancer diagnosis and year of birth, was used. Individual absorbed organ doses were calculated between 1986 and 2020 including external and internal exposure. Hazard ratios (HR) per mGy with 95% confidence intervals (95% CI) were calculated using conditional logistic regression adjusted for rural/nonrural habitat, education level and pre-Chernobyl cancer incidence 1980 to 1985. A total of 161,325 cancer cases in males and 144,439 in females were included.
    UNASSIGNED: The adjusted HR per mGy for all cancer sites combined was 1.027 (95% CI = 1.022, 1.031) in males and 1.011 (95% CI = 1.006, 1.017) in females. In a post hoc analysis accounting for both remaining confounding from hunter lifestyle and the pre-Chernobyl cancer incidence by county, the adjusted HR per mGy for all cancer sites combined was 1.014 (95% CI = 1.009, 1.019) in males and 1.000 (95% CI = 0.994, 1.006) in females. The post hoc analysis suggested an increased risk of cancer in the colon, pancreas, and stomach, respectively, in males, and lymphoma in females.
    UNASSIGNED: Increased cancer risk estimates were found for some specific cancer sites but remaining uncontrolled confounding due to hunter lifestyle could not be ruled out.
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  • 文章类型: Journal Article
    由于释放的放射性核素而发生核事故后,对环境的放射性污染是最大的威胁之一。从放射毒理学的角度来看,最重要的放射性核素是铯-137。主要是在核爆炸期间形成的,铯-137可以在土壤中持续多年,从那里它不断进入食物链。保障食品安全的一个要素是对其放射性污染的监测,主要是放射性铯同位素.该研究的目的是确定动物源性食品中铯137的含量。
    总共有1416个来自牛的肌肉样本,绵羊,猪,游戏和鱼,以及鸡蛋和乳制品使用伽马射线光谱法进行了检查。
    铯-137活性范围从低于最低可检测活性浓度(MDC)到超过4,000Bq/kg湿重(w.w.)。大多数情况下,这些值不超过MDC或在低于100Bq/kg的范围内。唯一的例外是游戏动物的肌肉组织,尤其是野猪,记录到铯137的显着活动,其中最高的是4,136.8±238Bq/kgw.w.为每个基质确定的有效剂量范围为0.01至0.83µSv/kg,为野猪确定的最高值。
    所计算的暴露剂量的值远低于公认的低辐射剂量(100mSv),并不表明所消耗的食物中存在任何大量的电离辐射。
    UNASSIGNED: Radioactive contamination of the environment is one of the greatest threats after a nuclear accident due to released radionuclides. From a radiotoxicological point of view, the most important radionuclide is caesium-137. Formed mainly during nuclear explosions, caesium-137 can persist in the soil for many years, from where it constantly enters the food chain. One of the elements of ensuring food safety is the monitoring of its radioactive contamination, mainly with radioactive caesium isotopes. The aim of the study was to determine the content of caesium-137 in food of animal origin.
    UNASSIGNED: A total of 1,416 muscle samples from cattle, sheep, pigs, game and fish, as well as chicken eggs and dairy products were examined using gamma-ray spectrometry.
    UNASSIGNED: Caesium-137 activities ranged from below the minimum detectable activity concentration (MDC) to over 4,000 Bq/kg wet weight (w.w.). Most often, the values did not exceed the MDC or were in a range below 100 Bq/kg. The exception was the muscle tissue of game animals, especially wild boar, where a significant activity of caesium-137 was recorded, the highest of which was 4,136.8 ± 238 Bq/kg w.w. Committed effective doses determined for each matrix ranged from 0.01 to 0.83 µSv/kg, with the highest value determined for wild boar.
    UNASSIGNED: The calculated exposure doses with values well below the accepted low radiation dose (100 mSv) did not indicate any significant amounts of ionising radiation from the food consumed.
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  • 文章类型: Journal Article
    UNASSIGNED:核设施周围的放射性监测对于为有效检测放射性泄漏到环境中提供重要的基线数据至关重要。我们旨在建立一项基线研究,以监测Sammen核电站(SNPP)周围90Sr和137Cs的放射性水平,并评估其对周围居民的健康影响。
    未经批准:在这项研究中,我们从2011年到2020年收集了SNPP周围的水和食物样本,并确定了90Sr和137Cs的活性浓度。我们统计分析了90Sr和137Cs的时间趋势,并评估了它们对当地居民的辐射暴露。
    未经评估:在此期间,水中90Sr和137Cs的活性浓度在1.2-9.9mBq/L和0.10-7.6mBq/L范围内变化,和0.037-1.3Bq/kg和0.011-0.45Bq/kg的食物,分别,无明显的季节变化趋势。
    UNASSIGNED:所有报告的90Sr和137Cs的活性浓度均显着低于WHO和中国国家标准的推荐值。由于SNPP在2018-2020年期间的运行,没有迹象表明研究区域有明显的放射性释放。摄入水和食物中90Sr和137Cs的年有效剂量(AED)远低于国际允许的限值,表明2011-2020年SNPP周围的辐射暴露保持在安全水平.
    Radioactivity monitoring around nuclear facilities is crucial to provide important baseline data for effective detection of radioactive leakage to the environment. We aim to establish a baseline study for monitoring radioactive levels of 90Sr and 137Cs around Sammen Nuclear Power Plant (SNPP) and to assess their associated health impact on surrounding residents.
    In this study, we collected water and food samples around the SNPP from 2011 to 2020 and determined for 90Sr and 137Cs activity concentrations. We statistically analyzed the temporal trends of 90Sr and 137Cs and evaluated their radiation exposure to the local residents.
    During this period, the activity concentrations of 90Sr and 137Cs varied within 1.2-9.9 mBq/L and 0.10-7.6 mBq/L in water, and 0.037-1.3 Bq/kg and 0.011-0.45 Bq/kg in food, respectively, with no significant seasonal variation trend.
    All reported activity concentrations of 90Sr and 137Cs were significantly lower than the recommended value of WHO and Chinese national standards. There is no indication of notable radioactive release into the study area due to the operation of SNPP during 2018-2020. The annual effective doses (AEDs) from the ingestion of 90Sr and 137Cs in water and food were well below the international permissible limits, indicating the radiation exposure around SNPP during 2011-2020 was kept at a safe level.
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  • 文章类型: Journal Article
    提供了2011年福岛第一核电站发生核事故后立即以气溶胶形式分散到环境中的129I大气活度浓度(以Bq/m3为单位)的数据。129I的放射性是在福岛和包括大都市在内的日本东部其他县的41个SPM监测点的滤带上收集的悬浮颗粒物(SPM)中确定的。用于通过加速器质谱(AMS)定量测定SPM样品中的129I,129I是化学分离的。在129I测量之前,使用Ge半导体探测器通过伽马射线光谱法确定相同SPM样品的137Cs活性。结合两种核素的活性浓度,计算每个SPM样品的129I/137Cs(Bq/Bq)的活性比。在我们的研究项目中,129I和137Cs的大气活度浓度,并获得920个SPM样品的活性比。与这些数据相关的科学讨论在题为“2011年福岛核事故后日本东部大气129I浓度和129I/137Cs比率的时间序列变化”的研究文章中进行了描述,日本\“(Ebihara等人。2022),其中提供了363个数据集。本文介绍了其余的557个数据集,所以这篇数据文章弥补了原始研究文章(Ebihara等人。2022年)。获得整个分析程序的空白值。此外,分析了试剂和过滤器(全新和使用过的过滤器)的试剂和过滤器,以评估这些样品对129I活性的贡献。这些数据也在本文中介绍。
    Data of the atmospheric activity concentrations (in Bq/m3) of 129I dispersed into the environment as aerosol immediately after the nuclear accident at Fukushima Daiichi Nuclear Power Plant in 2011 are presented. The radioactivity of 129I was determined in suspended particulate matter (SPM) collected on filter tapes at 41 SPM monitoring sites in Fukushima and other prefectures in eastern Japan including the metropolitan area. For quantitative determination of 129I in SPM samples by accelerator mass spectrometry (AMS), 129I was chemically separated. Prior to the 129I measurement, the 137Cs activity was determined for the same SPM sample by gamma-ray spectrometry using Ge-semiconductor detectors. Combining activity concentrations of the two nuclides, an activity ratio of 129I/137Cs (in Bq/Bq) was calculated for each SPM sample. In our research project, atmospheric activity concentrations of 129I and 137Cs, and their activity ratios were obtained for 920 SPM samples. Scientific discussion related to those data was described in the research article entitled \"Time-series variations of atmospheric 129I concentrations and 129I/137Cs ratios in eastern Japan just after the 2011 nuclear accident in Fukushima, Japan\" (Ebihara et al. 2022), where 363 data sets were presented. The remaining 557 data sets are presented in this article, so this data article makes up for the original research article (Ebihara et al. 2022). Blank values were obtained for whole analytical procedure. In addition, those for reagents and filters (both bland-new and used filters) were analyzed for assessing the contribution of the 129I activity from these samples. Those data also are presented in this article.
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  • 文章类型: Journal Article
    由于意外的核灾难和放射性元素的授权排放,放射性核素污染是一个令人担忧的威胁,无论是过去还是现在。使用原子能发电与未解决的有关残留物和污染物存储的问题有关。例如,1986年切尔诺贝利核事故和2011年福岛核事故导致土壤中铯(Cs)大量沉积,以及其他放射性核素。在Cs放射性变体中,人为放射性同位素137Cs(t½=30.16年)是严重的环境问题,由于其在衰变过程中迅速掺入生物系统并发射β和γ辐射。为了修复受污染的区域,大多数传统技术的应用是不环保的。因此,一种替代的绿色技术,即,植物修复,将来应该考虑和实施。这种可持续技术产生有限的二次废物,其目标是利用积累过多的植物来提取,稳定,降解,过滤放射性核素。该综述强调了植物吸收放射性核素的机制以及该过程中涉及的不同环境因素的影响,同时考虑其长期影响。
    Radionuclide contamination is a concerning threat due to unexpected nuclear disasters and authorized discharge of radioactive elements, both in the past and in present times. Use of atomic power for energy generation is associated with unresolved issues concerning storage of residues and contaminants. For example, the nuclear accidents in Chernobyl 1986 and Fukushima 2011 resulted in considerable deposition of cesium (Cs) in soil, along with other radionuclides. Among Cs radioactive variants, the anthropogenic radioisotope 137Cs (t½ = 30.16 years) is of serious environmental concern, owing to its rapid incorporation into biological systems and emission of β and γ radiation during the decaying process. To remediate contaminated areas, mostly conventional techniques are applied that are not eco-friendly. Hence, an alternative green technology, i.e., phytoremediation, should in future be considered and implemented. This sustainable technology generates limited secondary waste and its objectives are to utilize hyper-accumulating plants to extract, stabilize, degrade, and filter the radionuclides. The review highlights plant mechanisms for up-taking radionuclides and influences of different environmental factors involved in the process, while considering its long-term effects.
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  • 文章类型: Journal Article
    这项工作的目的是证明使用沉积在沉积物芯中的放射性核素来估算沉积条件,该沉积物芯取自被沼泽泥炭植被包围的过度生长的营养不良湖泊。沉积物岩心样品取自ToporoweStawy湖(Niñni(TSN)和Wyñni(TSW);塔特拉山脉)。使用Limnos取样器进行取样。物理样品制备后,进行伽马测量。进行了放射化学分析,目的是通过210Po测定210Pb的放射性。TSN湖的平均值如下:137Cs〜123Bq‧kg-1、40K〜389Bq‧kg-1、228Th〜55Bq‧kg-1、226Ra〜86Bq‧kg-1、241Am〜5Bq‧kg-1和210Pbuns〜180Bqkg-1。对于TSW湖,226Ra和241Am的放射性水平与TSN相当。137Cs的平均值,40K,228Th几乎是TSN的两倍。TSN最上层的210Pb水平高于TSW。沉积物采用210Pb方法测定,并估算了各层的沉降速率。基本化学计量学工具用于确认放射性核素的沉积方式,找到变量之间的相关性,并比较分析的湖泊。结论是,所提出的湖泊类型是有价值的信息来源,放射性核素的垂直分布可用于解释近150-200年来的物质供应来源和影响沉积过程的因素。
    The aim of this work was to prove the use of radionuclides deposited in sediment core taken from an overgrowing dystrophic lakes surrounded by marsh-peat vegetation to estimate sedimentary conditions. Sediment core samples were taken from the Toporowe Stawy Lakes (Niżni (TSN) and Wyżni (TSW); Tatra Mountains). The sampling was done using a Limnos corer. After the physical sample preparations, gamma measurements were performed. Radiochemical analysis was applied with the aim of determining 210Pb radioactivity by means of 210Po. The mean values for TSN lake are as follows: 137Cs ~ 123 Bq∙kg-1, 40 K ~ 389 Bq∙kg-1, 228Th ~ 55 Bq∙kg-1, 226Ra ~ 86 Bq∙kg-1, 241Am ~ 5 Bq∙kg-1, and 210Pbuns ~ 180 Bq∙kg-1. For TSW lake, the radioactivity levels of 226Ra and 241Am are comparable to the TSN. The mean values of 137Cs, 40 K, and 228Th are almost twice as high as in TSN. The level of 210Pb in uppermost layer of TSN is higher than in TSW. Sediments were dated by use of 210Pb method, and the rate of sedimentation of each layer was also estimated. Basic chemometric tools were used to confirm the way of deposition of radionuclide, find the correlations between variables, and compare analyzed lakes. It was concluded that the presented type of lakes are a valuable source of information and the vertical distribution of radionuclide can be used to interpret the source of material supply and factors that influence the sedimentation process in recent 150-200 years.
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  • 文章类型: Journal Article
    这项研究考虑了白俄罗斯受污染最严重的Gomel和Mogilev州的人口暴露于切尔诺贝利事故造成的长期辐射源。开发了剂量重建方法,并将其应用于这项研究中,以估计(i)来自地面上沉积的γ发射放射性核素的外部辐射和(ii)134Cs的红骨髓剂量(RBM)。137Cs和90Sr与当地生产的食品一起摄入。Gomel和Mogilev州的成年居民在切尔诺贝利事故后35年累积的平均人口加权RBM剂量分别为12和5.7mGy,分别,而最年轻年龄组的剂量降低了20-40%。1986-2021年,在Narovlya,成年人的平均区域特异性RBM剂量最高,分别为63、56和46mGy,Gomel州的Vetka和Korma地区,分别。对于大多数地区来说,外照射是暴露的主要途径(占总剂量的60-70%),除137Cs土壤对牛乳的聚集系数极高的地区外(≥5.0BqL-1/kBqm-2),其中134Cs和137Cs摄入对总RBM剂量的贡献超过70%。在Gomel和Mogilev州的大多数地区,90Sr摄入量对成人总RBM剂量的贡献不超过4%,新生儿不超过10%。本研究中估计的剂量的有效性是通过与1987-2015年热释光剂量计和全身计数器测量获得的剂量进行比较来评估的。本研究中开发的方法可用于计算除RBM以外的靶器官的剂量,例如甲状腺和乳腺剂量。本研究中估计的年龄依赖性和人口加权剂量对生态流行病学研究很有用,辐射风险的预测,以及对暴露于切尔诺贝利辐射的人群进行分析流行病学研究的理由。
    This study considers the exposure of the population of the most contaminated Gomel and Mogilev Oblasts in Belarus to prolonged sources of irradiation resulting from the Chernobyl accident. Dose reconstruction methods were developed and applied in this study to estimate the red bone-marrow doses (RBMs) from (i) external irradiation from gamma-emitting radionuclides deposited on the ground and (ii) 134Cs, 137Cs and 90Sr ingestion with locally produced foodstuffs. The mean population-weighted RBM doses accumulated during 35 years after the Chernobyl accident were 12 and 5.7 mGy for adult residents in Gomel and Mogilev Oblasts, respectively, while doses for youngest age groups were 20-40% lower. The highest mean area-specific RBM doses for adults accumulated in 1986-2021 were 63, 56 and 46 mGy in Narovlya, Vetka and Korma raions in Gomel Oblast, respectively. For most areas, external irradiation was the predominant pathway of exposure (60-70% from the total dose), except for areas with an extremely high aggregated 137Cs soil to cow\'s milk transfer coefficient (≥ 5.0 Bq L-1 per kBq m-2), where the contribution of 134Cs and 137Cs ingestion to the total RBM dose was more than 70%. The contribution of 90Sr intake to the total RBM dose did not exceed 4% for adults and 10% for newborns in most raion in Gomel and Mogilev Oblasts. The validity of the doses estimated in this study was assessed by comparison with doses obtained from measurements by thermoluminescence dosimeters and whole-body counters done in 1987-2015. The methodology developed in this study can be used to calculate doses to target organs other than RBM such as thyroid and breast doses. The age-dependent and population-weighted doses estimated in this study are useful for ecological epidemiological studies, for projection of radiation risk, and for justification of analytical epidemiological studies in populations exposed to Chernobyl fallout.
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  • 文章类型: Journal Article
    The vertical distribution of 137Cs in peat bog soils in the remote period after the Chernobyl Nuclear Power Plant accident (ChNPP, 1986) was investigated. The study was conducted on bog meadows in the Bryansk region of Russia. Soil samples were taken at 4 locations: 2 sites on lowland bogs and 2 sites on transitional bogs. Fifteen years after the accident, analysis of soils showed that the peak of 137Cs activity was still in the upper 10-cm layer. The highest percentage of the initial 137Cs deposition (92%) has been observed in the top 10-cm layer in the drained transitional bog. The lowest part of the initial 137Cs deposition (40%) has been found in 0-10-cm horizon in lowland bog with the deep peat layer. The findings revealed that elevated soil moisture promotes 137Cs downward migration. It was shown that ammonium has a major impact on mobility of 137Cs in bog soils. On average, the soil solution NH4+ concentrations exceeded the K+ concentrations by about a factor 5. A significant linear relationship was found between the rates of 137Cs removal from the top layers with the soil solution NH4+ concentrations.
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  • 文章类型: Journal Article
    There are no results of comparative ecological studies of the radionuclide activity concentration in the plants and soil in relation to geological substrate. Presented research encompasses the comparative analysis of the concentration of four radionuclides, three natural (40K, 226Ra, 232Th) and one artificial (137Cs) in soil samples and aerial plant parts of Teucrium montanum from different natural habitats on serpentinite and calcareous geological substrate. The activity concentrations of radionuclides were measured with high purity germanium (HPGe) detector and expressed as Bq kg-1. The calculated activity concentrations of 40K, 226Ra, 232Th, and 137Cs in soil samples from serpentinite/calcareous habitats are in range 39.6-91.0/59.3-1018.8, 1.7-5.5/4.3-52.4, 2.4-10.9/5.9-72.9, and 57.2-844.9/29.6-701.5 Bq kg-1, respectively. The activity concentrations of 40K, 226Ra, 232Th, and 137Cs in plant samples are in range 152.9-445.9/228.0-521.4, n.d.-1.2/0.6-5.6, n.d./0.2-0.9, and 1.0-46.4/1.7-7.0 Bq kg-1, respectively. The obtained results showed that the quantities of 137Cs are greater in the soil and plant material from the serpentinite habitats, while quantities of 40K, 226Ra, and 232Th are greater in the soil and plant material from calcareous habitats. In general, the level of radioactivity in plants and soil depends on the type of the geological substrate. The content of radionuclides in plants is correlated with the radionuclide content in the soil. In addition to other specifics in physical and chemical properties, serpentinite habitats are characterized by an increased amount of Cs in the soil, which causes an increased amount of this radionuclide in plants such as Teucrium montanum.
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