Water Pollution

水污染
  • 文章类型: Journal Article
    The COVID-19 pandemic\'s disruptions to human activities prompted serious environmental changes. Here, we assessed the variations in coastal water quality along the Caspian Sea, with a focus on the Iranian coastline, during the lockdown. Utilizing Chlorophyll-a data from MODIS-AQUA satellite from 2015 to 2023 and Singular Spectrum Analysis for temporal trends, we found a 22% Chlorophyll-a concentration decrease along the coast, from 3.2 to 2.5 mg/m³. Additionally, using a deep learning algorithm known as Long Short-Term Memory Networks, we found that, in the absence of lockdown, the Chlorophyll-a concentration would have been 20% higher during the 2020-2023 period. Furthermore, our spatial analysis revealed that 98% of areas experienced about 18% Chlorophyll-a decline. The identified improvement in coastal water quality presents significant opportunities for policymakers to enact regulations and make local administrative decisions aimed at curbing coastal water pollution, particularly in areas experiencing considerable anthropogenic stress.
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  • 文章类型: Journal Article
    最近在孔敬省进行的一项研究,泰国,评估了旨在改善水质和解决主要水体周围社区相关健康问题的技术辅助干预措施的有效性。该干预措施针对与水污染相关的健康问题,包括慢性肾病,皮肤状况,高血压,神经症状。该研究包括586名居民的水质评估和健康评估,并在13个社区实施了学习创新平台(LIP)。结果显示社区有显著改善,包括高血压和皮肤相关健康问题的减少,以及提高社区对实施简单水质评估和处理的认识和熟练程度。这项研究证明了全面的价值,技术驱动的社区方法,有效提高水质和健康结果,并在管理环境健康风险方面提高社区意识和自给自足。
    A recent study conducted in Khon Kaen Province, Thailand, evaluated the effectiveness of a technology-assisted intervention aimed at improving water quality and addressing related health issues in communities around key water bodies. The intervention targeted health concerns associated with water contamination, including chronic kidney diseases, skin conditions, hypertension, and neurological symptoms. The study included water quality assessments and health evaluations of 586 residents and implemented a Learning Innovation Platform (LIP) across 13 communities. Results showed significant improvements in the community, including a decrease in hypertension and skin-related health issues, as well as enhanced community awareness and proficiency in implementing simple water quality assessments and treatment. The study demonstrated the value of a comprehensive, technology-driven community approach, effectively enhancing water quality and health outcomes, and promoting greater community awareness and self-sufficiency in managing environmental health risks.
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  • 文章类型: Journal Article
    该研究旨在评估烟头过滤嘴(CBF)作为水中溶解有机碳(DOC)的潜在来源,从而形成消毒副产物。两种不同形式的CBF-完整(I)和分解(D),当它们发生在环境中时,选择在氯化(CI,CD)中浸出,非氯化(NI,ND),和高度氯化(HCD)水样。浸出液样品的紫外吸收曲线表明,完整的CBFs表现出更高的DOC浸出相比,分解的,在氯化样品中进一步加重(CI>CD>NI>ND)。浸出液的傅立叶变换红外光谱显示存在醋酸纤维素及其氯化衍生物的特征官能团,表明聚合物的潜在降解。此外,氯化样品中三卤甲烷(THM)的形成在CI样品中相对较高(2-11.5倍),与DOC浸出趋势一致。Further,CI和CD样品中不同THM的形态特征相似。尽管CI和CD样本的光谱和形态分析显示出可忽略的变化,HCD样品描绘了显著的表面粗糙度,其特征在于凹坑和孔的形成,随着结晶度的演变。这表明CBF的加速降解和乙酰基的破坏是氯浓度升高的一个因素。
    The study aimed to evaluate cigarette butt filters (CBFs) as a potential source of dissolved organic carbon (DOC) in water leading to the formation of disinfection by-products. Two different forms of CBFs - intact (I) and disintegrated (D), as they occur in the environment, were selected for leaching in chlorinated (CI, CD), non-chlorinated (NI, ND), and highly chlorinated (HCD) water samples. The UV absorbance profiles of the leachate samples showed that intact CBFs exhibited higher DOC leaching compared to the disintegrated ones, which was further accentuated in chlorinated samples (CI > CD > NI > ND). The Fourier Transform Infrared spectra of the leachates revealed the presence of characteristic functional groups of cellulose acetate and its chlorinated derivatives, indicating the potential degradation of the polymer. Moreover, trihalomethane (THM) formation in chlorinated samples was relatively higher in CI samples (2 - 11.5 times) compared to CD, consistent with the DOC leaching trends. Further, the speciation characteristics of different THMs in both CI and CD samples were similar. Although spectral and morphological analyzes of CI and CD samples revealed negligible variation, HCD samples depicted significant surface roughness characterized by the formation of pits and holes, along with the evolution of crystallinity. This suggested accelerated degradation of CBFs and disruption of acetyl groups as a factor of elevated chlorine concentrations.
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  • 文章类型: Journal Article
    迫切需要解决铬污染的工业废水带来的严重环境风险,因此需要开发环保的清洁方法。利用榕属植物提取物,本研究旨在开发绿色纳米氧化锌用于去除废水中的Cr金属离子。无花果的叶子,通常被称为榕树,用于提取用于合成ZnONP的溶液。开发这些纳米颗粒的目的是有效地从工业废水中消除铬(Cr)。进行了批量研究,以评估这些合成的ZnONPs在处理皮革工业废水中的效率,旨在实现最佳的铬去除。这涉及通过比较处理前后的铬水平来测量纳米颗粒从废水样品中吸附Cr离子的能力。通过优化pH等批次来估算Cr的去除效率,接触时间,ZnONPs的初始Cr浓度和吸附剂剂量为批次。发现这些合成的ZnONP成功地降低了废水中的铬含量以达到允许的极限。纳米粒子表现出最高的吸收能力,在pH为4时达到94%(46mg/g),接触时间为7小时,最佳吸附剂剂量为0.6g/L。因此,这些纳米粒子优异的吸附能力,加上他们对环境无害的制造技术,为铬污染废水处理提供长期高效的解决方案。其新颖的性质具有显着提高水生态系统的安全性和清洁度的潜力,保护人类健康和环境。
    The urgent need to address the severe environmental risk posed by chromium-contaminated industrial wastewater necessitates the development of eco-friendly cleanup methodologies. Utilizing the Ficus benghalensis plant extracts, the present study aims to develop green zinc oxide nanoparticles for the removal of Cr metal ions from wastewater. The leaves of Ficus benghalensis, often known as the banyan tree, were used to extract a solution for synthesizing ZnO NPs. These nanoparticles were developed with the goal of efficiently eliminating chromium (Cr) from industrial effluents. Batch studies were carried out to assess the efficiency of these synthesized ZnO NPs in treating leather industrial effluent, with aiming for optimal chromium removal. This involved measuring the nanoparticles\' capacity to adsorb Cr ions from wastewater samples by comparing chromium levels before and after treatment. Removal efficiency for Cr was estimated through the batches such as optimization of pH, contact time, initial Cr concentration and sorbent dose of ZnO NPs were of the batches. These synthesized ZnO NPs were found to be successful in lowering chromium levels in wastewater to meet permissible limit. The nanoparticles exhibited their highest absorption capacity, reaching 94 % (46 mg/g) at pH 4, with a contact time of 7 hours with the optimum sorbent dose of 0.6 g/L. Hence, the excellent adsorption capabilities of these nanoparticles, together with their environmentally benign manufacturing technique, provide a long-term and efficient solution for chromium-contaminated wastewater treatment. Its novel nature has the potential to significantly improve the safety and cleanliness of water ecosystems, protecting the both i.e. human health and the environment.
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  • 文章类型: Journal Article
    公众参与对于提高水治理系统的绩效至关重要,特别是在自上而下的层次结构主导的治理模式中。公众关注,作为公众参与的重要形式,被认为是促进水治理的重要组成部分。然而,很少有研究探讨不同的公众关注导致不同的水治理结果的不同影响。本研究通过探索与水相关的公众关注对水污染控制和政府污染缓解行动的直接和间接影响来解决这一差距。使用从中国社交媒体抓取的公民与水有关的帖子。结果表明,与水有关的公众关注通过其对减少水污染的直接影响和通过促进政策行动的间接影响来促进水治理。具体来说,与水污染危害有关的担忧,水污染监测,预防产品,与其他类型的关注相比,水污染控制措施对减少水污染有更积极的影响。同时,公众的担忧在触发与经济相关和与基础设施相关的水污染缓解行动方面表现出更强的影响。这项研究提供了细致入微的见解,以了解公众参与在改善水治理中的作用,其调查结果对通过自下而上的方法加强水治理系统的问责制具有深刻的见解。
    Public participation is crucial to improving the performance of water governance systems, especially in a governance model dominated by a top-down hierarchical structure. Public concerns, as a vital form of public participation, have been acknowledged as an essential component in contributing to water governance. However, few studies explore the varying effects of diverse public concerns in leading to different water governance outcomes. This study addresses this gap by exploring the direct and indirect effects of water-related public concerns on water pollution control and governments\' pollution mitigating actions, using citizens\' water-related posts crawled from China\'s social media. Results show that public water-related concerns contribute to water governance both through its direct effects on reducing water pollution and indirect effects by promoting policy actions. Specifically, the concerns related to water pollution hazards, water pollution monitoring, prevention products, and water pollution control measures have more positive impacts on water pollution reduction compared to other types of concern. Meanwhile, public concerns demonstrate stronger effects in triggering economic-related and infrastructure-related water pollution mitigation actions. This study provides nuanced insights to understand the role of public participation in improving water governance, the findings of which are insightful to enhance accountability of water governance systems through a bottom-up approach.
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  • 文章类型: Journal Article
    心血管疾病是全球死亡的重要原因,和他们的流行可以被一系列的环境因素放大。这篇综述文章批判性地评估了已发表的有关各种环境因素的流行病学和病理生理机制的信息,例如空气室内和室外空气污染,水污染,气候变化,和土壤污染。讨论了减轻这些影响的预防措施,包括公共卫生对策,并在我们对未来研究的知识中存在差距。
    Cardiovascular diseases are a significant cause of mortality worldwide, and their prevalence can be amplified by a range of environmental factors. This review article critically evaluated the published information on the epidemiology and pathophysiological mechanisms of various environmental factors such as air indoor and outdoor air pollution, water pollution, climate change, and soil pollution. Preventative measures to mitigate these effects including public health responses are discussed with gaps in our knowledge for future studies.
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  • 文章类型: Journal Article
    在全球范围内,水生生态系统中的锑(Sb)污染已成为关键的环境问题。强调迫切需要具有成本效益和用户友好的技术从水源中去除Sb化合物。在这项研究中,一种新型吸附剂,硒纳米颗粒(SeNPs),是使用PsidiumguajavaL.叶的水提取物(AEP)合成的,目的是从水溶液中消除Sb(III)。使用扫描电子显微镜(SEM)表征生物合成的SeNPs,能量色散X射线光谱(EDS),X射线荧光光谱仪(XRF),傅里叶变换红外(FT-IR)光谱,X射线衍射(XRD)拉曼光谱和X射线光电子能谱(XPS)剖析技巧。此外,在SeNPs剂量的影响下,系统研究了SeNPs对Sb(III)的去除效率,温度,pH值和可重用性。研究结果表明,吸附数据很好地拟合了伪二阶模型,而Sips模型证明了SeNPs在303.15K时对水溶液中Sb(III)离子的高吸附能力(62.7mg/g)。-22.59kJ/mol的放热焓变化和负吉布斯自由能变化确保了在所考虑的温度条件下吸附过程的可行性。SeNP上的表面官能团,如羧基,酰胺,羟基,羰基,和亚甲基显著促进吸附过程。此外,两个实际的Sb矿山废水样品中Sb的去除效率非常高,在48小时内使用1.5g/L的SeNPs达到近100%。这一结果强调了SeNPs作为高效修复来自水生环境的Sb的非常有前途的解决方案的潜力,由于其成本效益,易于再生,和快速摄取能力。
    Antimony (Sb) pollution in aquatic ecosystems has emerged as a critical environmental issue on a global scale, emphasizing the urgent need for cost-effective and user-friendly technologies to remove Sb compounds from water sources. In this study, a novel adsorbent, selenium nanoparticles (SeNPs), was synthesized using the aqueous extract of Psidium guajava L. leaves (AEP) for the purpose of eliminating Sb(III) from aqueous solutions. The biosynthesized SeNPs was characterized using scanning electron microscopy (SEM), energy dispersive X-ray spectroscopy (EDS), X-ray fluorescence spectrometer (XRF), Fourier Transform-Infrared (FT-IR) spectroscopy, X-ray diffraction (XRD), Raman spectroscopy and X-ray photoelectron spectroscopy (XPS) analysis techniques. Additionally, the removal efficiency of the SeNPs for Sb(III) was systematic investigated under the effects of SeNPs dose, temperature, pH and re-usability. The results of this study showed that the adsorption data fitted well into pseudo-second order model, while the Sips modeling demonstrated a high adsorption capacity (62.7 mg/g) of SeNPs for Sb(III) ions at 303.15 K from aqueous solution. The exothermic enthalpy change of - 22.59 kJ/mol and negative Gibbs free energy change assured the viability of the adsorption process under the considered temperature conditions. Surface functional groups on SeNPs like carboxyl, amide, hydroxyl, carbonyl, and methylene significantly facilitate the adsorption processes. Furthermore, the removal efficiencies of Sb in the two actual Sb mine wastewater samples were remarkably high, achieving nearly to 100% with 1.5 g/L SeNPs within 48 h. This outcome underscores the potential of SeNPs as a highly promising solution for efficiently remediating Sb from aquatic environments, owing to their cost-effectiveness, ease of regeneration, and rapid uptake capabilities.
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  • 文章类型: Journal Article
    尼古丁是香烟烟雾中捕获在过滤器中的主要污染物之一。烟蒂的尼古丁泄漏是与这种危险废物相关的问题之一。在这项研究中,在降雨等三个参数的影响下,研究了烟头泄漏到城市环境中的尼古丁浓度,密度,以及散落的烟头的耐用性。根据城市环境中烟头耐久性的差异和湿度比,在六种情况下估算了尼古丁向环境中的泄漏。结果表明,垃圾烟头的密度为0.0019-0.294数量/m2。住宅用地中乱扔烟头的密度比商业用地低52.38%。尼古丁从烟头泄漏在商业,住宅,休闲用地分别为1.1、0.484和.0065mg/m2。在研究的场景中,在最好和最坏的情况下,335,070和481,950克/年的尼古丁将从烟头泄漏到水资源中。考虑到烟头是包括尼古丁在内的毒素对环境的严重来源,有必要采取控制措施来降低其在城市环境中的密度。
    Nicotine is one of the main pollutants in cigarette smoke that trapped in the filter. Nicotine leakage from cigarette butts is one of the concerns associated with this hazardous waste. In this study, the concentration of nicotine leaked from cigarette butts into the urban environment was investigated under the influence of three parameters including rainfall, density, and the durability of the littered cigarette butt. The leakage of nicotine into the environment was estimated in six scenarios based on the difference in the durability of cigarette butts in the urban environment and the humidity ratio. The results showed that the density of littered cigarette butts was 0.0019-0.294 number/m2. The density of littered cigarette butts in residential land-use was 52.38% lower than commercial land-use. Nicotine leakage from cigarette butts in commercial, residential, and recreational land-uses was 1.1, 0.484, and .0065 mg/m2, respectively. In the studied scenarios, in the best and worst case, 335,070 and 481,950 gr/year of nicotine will leak from the cigarette butt into the water resources. Considering that cigarette butts are a serious source of toxins including nicotine to the environment, control measures are necessary to reduce its density in the urban environment.
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  • 文章类型: Journal Article
    由于过量使用,兽用抗生素已成为水和废水来源中的新兴污染物,对传统水和废水处理的毒性和抗性。本研究探索了使用Ti-RuO2/IrO2阳极的电化学氧化(EO)降解模型抗生素-氟苯尼考(FF)。使用SEM-EDS研究对阳极材料进行了表征,该研究表明了相邻金属氧化物之间的稳定结构和最佳相互作用。EDS结果显示Ru的存在,Ir,Ti,O和C元素占6.44%,2.57%,9.61%,52.74%和28.64%的原子重量百分比,分别。优化研究表明,pH5,30mAcm-2电流密度和0.05MNa2SO4对于5mgL-1FF在360分钟的处理时间内达到了90%的TOC去除率。降解遵循伪一级动力学。LC-Q-TOF-MS研究揭示了六种主要的副产物,说明了羟基化,放气,脱氯是FF电化学氧化过程中的主要降解机理。离子色谱研究显示Cl-的增加,F-和NO3-离子随着治疗时间的推移,在治疗的初始阶段后,Cl-减少。使用斑马鱼(Daniorerio)幼虫进行的毒性研究表明,处理过的样品具有毒性,可诱发发育障碍,例如心包水肿,卵黄囊水肿,受精后96小时(hpf)的脊柱弯曲和尾巴畸形。与控制相比,在处理的胚胎中观察到延迟的孵化和凝固。总的来说,这项研究为了解混合金属氧化物(MMO)阳极对使用电化学氧化降解兽用抗生素污染的水和废水源的影响奠定了基础。
    Veterinary antibiotics have become an emerging pollutant in water and wastewater sources due to excess usage, toxicity and resistance to traditional water and wastewater treatment. The present study explored the degradation of a model antibiotic- Florfenicol (FF) using electrochemical oxidation (EO) with Ti-RuO2/IrO2 anode. The anode material was characterized using SEM-EDS studies expressing stable structure and optimal interaction of the neighboring metal oxides with each other. The EDS results showed the presence of Ru, Ir, Ti, O and C elements with 6.44%, 2.57%, 9.61%, 52.74% and 28.64% atomic weight percentages, respectively. Optimization studies revealed pH 5, 30 mA cm-2 current density and 0.05 M Na2SO4 for 5 mg L-1 FF achieved 90% TOC removal within 360 min treatment time. The degradation followed pseudo-first order kinetics. LC-Q-TOF-MS studies revealed six predominant byproducts illustrating hydroxylation, deflourination, and dechlorination to be the major degradation mechanisms during the electrochemical oxidation of FF. Ion chromatography studies revealed an increase in Cl-, F- and NO3- ions as treatment time progressed with Cl- decreasing after the initial phase of the treatment. Toxicity studies using Zebrafish (Danio rerio) embryo showed the treated sample to be toxic inducing developmental disorders such as pericardial edema, yolk sac edema, spinal curvature and tail malformation at 96 h post fertilization (hpf). Compared to control, delayed hatching and coagulation were observed in treated embryos. Overall, this study sets the stage for understanding the effect of mixed metal oxide (MMO) anodes on the degradation of veterinary antibiotic-polluted water and wastewater sources using electrochemical oxidation.
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  • 文章类型: Letter
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