Spatio-temporal variations

  • 文章类型: Journal Article
    在全球湖泊富营养化激增之际,调查和分析湖泊的水质和趋势对于制定有效的湖泊管理政策至关重要。水质指数(WQI)是通过整合来自多个水质参数的数据来评估水质的最常用工具之一。在这项研究中,我们分析了最大的高原湖泊之一的11个水质参数的时空变化,洱海,基于2014年1月至2021年12月的调查。利用机器学习模型,我们测量了不同水质参数对WQI的相对重要性,并进一步利用逐步多元线性回归得出最佳最小水质指数(WQImin),该指数需要最少数量的水质参数而不影响性能。我们的研究结果表明,洱海的水质通常呈改善趋势,如WQI表现的Mann-Kendall检验阳性所示(Z=2.89,p<0.01)。在五种机器学习模型中,XGBoost表现最好(确定系数R2=0.822,均方误差=3.430,平均绝对误差=1.460)。在11个水质参数中,只有四个(即,溶解氧,氨氮,总磷,和总氮)是最佳WQImin所需的。WQImin的建立有助于降低未来洱海水质监测的成本,这也可以作为在类似水域进行有效水质监测的有价值的框架。此外,对洱海水质时空格局和趋势的阐明为当局提供了指南针,提供见解,以支持未来的湖泊管理策略。
    Amid the global surge of eutrophication in lakes, investigating and analyzing water quality and trends of lakes becomes imperative for formulating effective lake management policies. Water quality index (WQI) is one of the most used tools to assess water quality by integrating data from multiple water quality parameters. In this study, we analyzed the spatio-temporal variations of 11 water quality parameters in one of the largest plateau lakes, Erhai Lake, based on surveys from January 2014 to December 2021. Leveraging machine learning models, we gauged the relative importance of different water quality parameters to the WQI and further utilized stepwise multiple linear regression to derive an optimal minimal water quality index (WQImin) that required the minimal number of water quality parameters without compromising the performance. Our results indicated that the water quality of Erhai Lake typically showed a trend towards improvement, as indicated by the positive Mann-Kendall test for WQI performance (Z = 2.89, p < 0.01). Among the five machine learning models, XGBoost emerged as the best performer (coefficient of determination R2 = 0.822, mean squared error = 3.430, and mean absolute error = 1.460). Among the 11 water quality parameters, only four (i.e., dissolved oxygen, ammonia nitrogen, total phosphorus, and total nitrogen) were needed for the optimal WQImin. The establishment of the WQImin helps reduce cost in future water quality monitoring in Erhai Lake, which may also serve as a valuable framework for efficient water quality monitoring in similar waters. In addition, the elucidation of spatio-temporal patterns and trends of Erhai Lake\'s water quality serves as a compass for authorities, offering insights to bolster lake management strategies in the future.
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  • 文章类型: Journal Article
    海水中叶绿素a(Chl-a)的浓度反映了浮游植物的生长和水体富营养化,通常对其进行评估,以评估珊瑚礁的初级生产力和碳源/汇。然而,当利用低空间分辨率的海洋卫星时,精确划定珊瑚礁中Chl-a浓度仍然是一个挑战。在这项研究中,在边缘礁中建立了Chl-a的遥感反演模型(R2=0.76,RMSE=0.41μg/L,MRE=14%)和环礁(R2=0.79,RMSE=0.02μg/L,MRE=8%),利用空间分辨率为30m的Landsat-8作战陆地成像仪(OLI)敏感波段的反射率数据。利用上述模型反演了2013年至2022年南海六个主要珊瑚礁地区Chl-a浓度的高分辨率分布图,随后用于分析Chl-a浓度的变化及其影响因素。结果表明,大亚湾珊瑚礁之间存在Chl-a浓度梯度,渭洲岛,鹿怀头,徐闻,黄岩岛,和西沙岛的顺序。珊瑚礁中Chl-a浓度总体呈上升趋势,有明显的季节性波动,其特征是冬季和春季浓度较高,夏季和秋季浓度较低。珊瑚礁中Chl-a的浓度与平均风速呈正相关。
    The concentration of chlorophyll-a (Chl-a) in seawater reflects phytoplankton growth and water eutrophication, which are usually assessed for evaluation of primary productivity and carbon source/sink of coral reefs. However, the precise delineation of Chl-a concentration in coral reefs remains a challenge when ocean satellites with low spatial resolution are utilized. In this study, a remote sensing inversion model for Chl-a was developed in fringing reefs (R2 = 0.76, RMSE =0.41 μg/L, MRE = 14 %) and atolls (R2 = 0.79, RMSE =0.02 μg/L, MRE = 8 %), utilizing reflectance data from the sensitive band of the Landsat-8 Operational Land Imagers (OLI) with a spatial resolution of 30 m. The aforementioned model was utilized to invert high-resolution distribution maps of Chl-a concentration in six major coral reef regions of the South China Sea from 2013 to 2022 and subsequently used to analyze the variations in Chl-a concentration and its influencing factors. The results indicate a Chl-a concentration gradient among coral reefs Daya Bay, Weizhou Island, Luhuitou, Xuwen, Huangyan Island, and Xisha Island in that order. The Chl-a concentration in coral reefs exhibited an overall increasing trend, with significant seasonal fluctuations, characterized by higher concentrations during winter and spring and lower concentrations during summer and autumn. The concentration of Chl-a in coral reefs was positively correlated with the average wind speed.
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  • 文章类型: Journal Article
    水污染事件已成为重大的生态和环境威胁,特别是关于饮用水水源地(DWSA)的安全。本研究旨在通过将地理信息系统(GIS)集成到使用C和FORTRAN编程语言开发的二维水动力水质数学模型中来解决此问题。重点是河上山饮用水水源地(HDWSA),TECPLOT360软件用于可视化污染物迁移和扩散过程。该研究特别考虑了假设的铅(Pb)污染事故,位于三峡库区(TGRA)。分析了整个DWSA中Pb浓度的时空变化,并对不同水季Pb浓度变化进行了比较。结果表明,在事故中,干旱季节取水时的Pb浓度,衰落季节,汛期,蓄水季节在76、58、44和48分钟达到标准极限,分别。此外,在各个季节中,整个DWSA在124、89、71和74分钟达到了标准的Pb浓度水平。该研究还观察到DWSA中Pb污染区的扩张和随后的收缩,Pb浓度的转移率排序为汛期>蓄水期>衰退期>旱季。
    Water contamination incidents have become a significant ecological and environmental threat, particularly concerning the security of drinking water source areas (DWSAs). This research aimed to address this issue by integrating Geographic Information System (GIS) into bidimensional hydrodynamic water quality mathematical model developed using C +  + and FORTRAN programming languages. The focus was on the Heshangshan drinking water source area (HDWSA), and the TECPLOT360 software was utilized for visualizing pollutant migration and dispersion processes. The study specifically considered a hypothetical lead (Pb) contamination accident, which is situated in the Three Gorges Reservoir Area (TGRA). The spatio-temporal variations in Pb concentration throughout the entire DWSA were analyzed, along with a comparison of Pb concentration changes during different water seasons. The results indicate that, during the accident, the Pb concentration at the water intake in the drought season, decline season, flood season, and impounding season reached the standard limits at 76, 58, 44, and 48 min, respectively. Moreover, the entire DWSA achieved standard levels of Pb concentration at 124, 89, 71, and 74 min during the respective seasons. The study also observed an expansion and subsequent contraction of the Pb contamination area in the DWSA, with the transfer rate of Pb concentration ranked as flood season > impounding season > decline season > drought season.
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  • 文章类型: Journal Article
    汞(Hg)对生态系统和人类健康的有害影响已得到充分证明。尽管发达国家报告了电子废物回收产生的气态元素汞(GEM)的排放,人们对全球南方的情况知之甚少。使用总共132个被动空气采样器,在2020年9月至2021年12月期间,在巴基斯坦的32个非正式电子废物回收设施和背景地点连续测量了空气中GEM的季节性浓度。研究地点的年平均GEM浓度范围为1.8至92ngm-3。在研究的城市中,在卡拉奇测量到更高的浓度(平均值±s。d:17±22,范围:4.2-92ngm-3),拉合尔(16±4.2,8.2-22ngm-3)和白沙瓦(15±17,4.9-80ngm-3),而在海德拉巴测量的水平较低(6.9±6.2,3.1-25ngm-3),与大都市地区非正式回收活动的比率更高一致。季节性,秋季(15±16:3.3-92ngm-3)和夏季(13±8.7:1.8-80ngm-3)的GEM水平高于冬季(12±8.4:2.5-49ngm-3)和春季(9.2±7.3:1.8-80ngm-3),可能反映了在较高温度下的挥发增强和/或不同季节的回收操作幅度不同。应在该国紧急制定和实施与电子废物管理有关的政策和严格法规。
    Detrimental effects of mercury (Hg) on ecosystems and human health have been well-documented. Whereas emissions of gaseous elemental mercury (GEM) from e-waste recycling have been reported in developed countries, much less is known about the situation in the Global South. Using a total of 132 passive air samplers, seasonally resolved concentrations of GEM in air were measured continuously at 32 informal e-waste recycling facilities and background location in Pakistan for a period of one year between September 2020 and December 2021. Annual average GEM concentrations at the studied locations ranged from 1.8 to 92 ng m-3. Among the studied cities, higher concentrations were measured in Karachi (mean ± s.d: 17 ± 22, range: 4.2-92 ng m-3), Lahore (16 ± 4.2, 8.2-22 ng m-3) and Peshawar (15 ± 17, 4.9-80 ng m-3), while lower levels were measured in Hyderabad (6.9 ± 6.2, 3.1-25 ng m-3), consistent with a higher rate of informal recycling activities in metropolitan areas. Seasonally, higher GEM levels occurred during autumn (15 ± 16: 3.3-92 ng m-3) and summer (13 ± 8.7: 1.8-80 ng m-3) than in winter (12 ± 8.4: 2.5-49 ng m-3) and spring (9.2 ± 7.3: 1.8-80 ng m-3), possibly reflecting enhanced volatilization at higher temperatures and/or varying magnitude of recycling operations in different seasons. Policies and strict regulations related to e-waste management should be developed and implemented urgently in the country.
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  • 文章类型: Journal Article
    在全球变暖的背景下,频繁发生的热浪灾害严重威胁着人类的生命财产安全。城市群,作为人口和经济高度集中的主要地区,由于现有的城市热岛效应,容易受到热编织的影响。在这项研究中,我们研究了热浪的时空特征(热指数,HI)在中国2000-2020年,并从暴露的角度评估了19个城市群对热浪的脆弱性,敏感性和适应性。结果表明:(1)在过去的20年里,HI的频率和强度(大于26.67°C)均呈上升趋势。(2)山东半岛,河南中部,长江三角洲,长江中游,辽宁中南部城市群始终保持较高的脆弱性。(3)从2000年到2020年,京津冀的脆弱性,长江三角洲,成都-重庆,长江中游,广东-福建-浙江,哈尔滨-长春和辽宁中南部城市群始终以暴露为主。山东半岛的脆弱性,北部湾和豫中城市群一直以敏感性为主。北天山的脆弱性,兰州-西宁,关中和湖宝鄂渝城市群一直以适应性不足为主导。(4)最近,造成暴露的因素最多,敏感性和适应性是人口密度,户外工人和供水的比例,贡献率为38%,55%和26%,分别。本研究可为城市群间资源的合理配置提供科学依据,有效制定政策,引导人口从高温灾害中迁移。
    In the context of global warming, frequent heat wave disasters have seriously threatened the safety of human life and property. The urban agglomeration, as the main region with a high concentration of population and economy, is susceptible to heat weaves due to the existing urban heat island effect. In this study, we investigated the temporal and spatial characteristics of heat waves (heat index, HI) in China from 2000 to 2020 and assess the vulnerability of 19 urban agglomerations to heat waves from the perspective of exposure, sensitivity and adaptability. The results show that: (1) In the past 20 years, the frequency and intensity of HI (greater than 26.67 °C) both showed an upward trend. (2) Shandong Peninsula, Central Henan, Yangtze River Delta, Middle Reaches of Yangtze River, and Mid-southern Liaoning urban agglomerations always maintain a high vulnerability. (3) From 2000 to 2020, the vulnerability of Beijing-Tianjin-Hebei, Yangtze River Delta, Chengdu-Chongqing, Middle reaches of Yangtze River, Guangdong-Fujian-Zhejiang, Harbin-Changchun and Mid-southern Liaoning urban agglomerations were always dominated by exposure. The vulnerability of Shandong Peninsula, Beibu Gulf and Central Henan urban agglomeration has always been dominated by sensitivity. The vulnerability of North Tianshan Mountain, Lanzhou-Xining, Guanzhong and Hu-Bao-E-Yu urban agglomeration has always been dominated by inadequate adaptability. (4) Recently, the factors that contributed most to exposure, sensitivity and adaptability were population density, the proportion of outdoor workers and water supply, with contribution rates of 38%, 55% and 26%, respectively. This study can provide a scientific basis for the rational allocation of resources among urban agglomerations, effectively formulating policies and guiding population migration from high temperature disasters.
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  • 文章类型: Journal Article
    时空特征,与气象因素的关系,和空气污染物的来源分布(2017年1月-2021年12月)进行了分析,以更好地了解新疆天山北坡(NSTM)的空气污染物,重工业污染严重的城市群。结果表明,SO2、NO2、CO、O3,PM2.5和PM10分别为8.61-13.76μgm-3,26.53-36.06μgm-3,0.79-1.31mgm-3,82.24-87.62μgm-3,37.98-51.10μgm-3和84.15-97.47μgm-3。大气污染物浓度(除O3外)呈下降趋势。浓度最高的是在冬天,在五家渠,石河子,昌吉,乌鲁木齐,还有吐鲁番,冬季颗粒物的浓度超过NAAQSII级。西风和局部污染物的扩散都对高浓度产生了实质性影响。根据对冬季后退轨迹的分析,气团主要来自哈萨克斯坦东部和当地的排放源,气流中的PM10对吐鲁番的影响较为显著;其余城市受PM2.5影响较大。潜在来源包括乌鲁木齐-昌吉-石河子,吐鲁番,北部巴音郭勒蒙古自治州,哈萨克斯坦东部。因此,改善空气质量的重点应该是减少本地排放,加强区域合作,研究空气污染物的越境迁移。
    The spatiotemporal characteristics, relationship with meteorological factors, and source distribution of air pollutants (January 2017-December 2021) were analyzed to better understand the air pollutants on the northern slope of the Tianshan Mountains (NSTM) in Xinjiang, a heavily polluted urban agglomeration of heavy industries. The results showed that the annual mean concentrations of SO2, NO2, CO, O3, PM2.5, and PM10 were 8.61-13.76 μg m-3, 26.53-36.06 μg m-3, 0.79-1.31 mg m-3, 82.24-87.62 μg m-3, 37.98-51.10 μg m-3, and 84.15-97.47 μg m-3. The concentrations of air pollutants (except O3) showed a decreasing trend. The highest concentrations were in winter, and in Wujiaqu, Shihezi, Changji, Urumqi, and Turpan, the concentrations of particulate matter exceeded the NAAQS Grade II during winter. The west wind and the spread of local pollutants both substantially impacted the high concentrations. According to the analysis of the backward trajectory in winter, the air masses were mainly from eastern Kazakhstan and local emission sources, and PM10 in the airflow had a more significant impact on Turpan; the rest of the cities were more affected by PM2.5. Potential sources included Urumqi-Changj-Shihezi, Turpan, the northern Bayingol Mongolian Autonomous Prefecture, and eastern Kazakhstan. Consequently, the emphasis on improving air quality should be on reducing local emissions, strengthening regional cooperation, and researching transboundary transport of air pollutants.
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  • 文章类型: Journal Article
    净生态系统生产力(NEP),在碳循环中起着关键作用,是生态系统碳收支的重要指标。在本文中,新疆自治区NEP的时空变化,基于遥感和气候再分析数据,对中国2001-2020年的数据进行了研究。改进的卡内基·艾姆斯·斯坦福方法(CASA)模型被用来估计净初级生产力(NPP),利用土壤异养呼吸模型计算土壤异养呼吸。然后通过计算NPP和异养呼吸之间的差异获得NEP。研究区的年平均NEP东部高西部低,北部高,南部低。研究区20年平均植被NEP为128.54gC·m-2,表明研究区总体上是碳汇。从2001年到2020年,年平均植被NEP介于93.12和158.05gC·m-2之间,并且总体上呈增加趋势。71.46%的植被面积表现出NEP的增加趋势。NEP与降水呈正相关,与气温呈负相关,与气温的相关性更为显著。该工作揭示了新疆自治区NEP的时空动态,可为评估区域固碳能力提供有价值的参考。
    Net ecosystem productivity (NEP), which plays a key role in the carbon cycle, is an important indicator of the ecosystem\'s carbon budget. In this paper, the spatial and temporal variations of NEP over Xinjiang Autonomous Region, China from 2001 to 2020 were studied based on remote sensing and climate re-analysis data. The modified Carnegie Ames Stanford Approach (CASA) model was employed to estimate net primary productivity (NPP), and the soil heterotrophic respiration model was used to calculate soil heterotrophic respiration. Then NEP was obtained by calculating the difference between NPP and heterotrophic respiration. The annual mean NEP of the study area was high in the east and low in the west, high in the north and low in the south. The 20-year mean vegetation NEP of the study area is 128.54 gC·m-2, indicating that the study area is a carbon sink on the whole. From 2001 to 2020, the annual mean vegetation NEP ranged between 93.12 and 158.05 gC·m-2, and exhibited an increasing trend in general. 71.46% of the vegetation area showed increasing trends of NEP. NEP exhibited a positive relationship with precipitation and a negative relationship with air temperature, and the correlation with air temperature was more significant. The work reveals the spatio-temporal dynamics of NEP in Xinjiang Autonomous Region and can provide a valuable reference for assessing regional carbon sequestration capacity.
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  • 文章类型: Journal Article
    东北地区种植了很多春玉米(辽宁,吉林,和黑龙江),极易干旱的地区。这里,利用中分辨率成像光谱辐射计数据的8天地表反射率和地表温度,研究了2002-2020年的遥感指标。使用决策树分类提取春玉米分布,并根据现场调查数据和公布的统计数据将结果与已知分布进行比较。结果表明,春玉米和大豆混合像素对春玉米时空变异研究的影响有限,错误是可以接受的。2018年至2020年春玉米分布验证总体准确率在85%以上。稳定的,波动,春玉米低频种植面积占11.86%,17.41%,和34.86%的研究区域,分别。2015年,政府指示减少东北“连道湾”地区的春玉米种植面积。春玉米种植面积在这一变化前呈现持续增长的特点(2002-2014年),表现出响应变化的变化和减少(2015-2017年),并在本次变更后(2018-2020年)表现出优化和恢复。与波动和低频种植面积相比,稳定种植区的中度和重度干旱较高。从2002年到2020年,最严重的干旱发生在扩大的种植区。这种对春玉米时空变化和干旱的快速大规模监测为提高籽粒产量提供了基础。该方法可以方便地应用于其他地区的研究,并与高分辨率和高光谱卫星数据相结合,以提高监测精度。
    A lot of spring maize is grown in Northeast China (Liaoning, Jilin, and Heilongjiang), an area that is highly susceptible to drought. Here, remote sensing indexes from 2002 to 2020 were studied using the 8-day surface reflectance and land surface temperature of Moderate-resolution Imaging Spectroradiometer data. Spring maize distribution was extracted using a decision tree classification, and the results were compared to the known distribution based on field investigation data and published statistics. The results showed that mixed pixels of spring maize and soybeans had limited influence on the study of spatio-temporal variations of spring maize, and the error was acceptable. The overall accuracy of verifying the spring maize distribution from 2018 to 2020 was above 85%. The stable, fluctuating, and low-frequency planting areas of spring maize accounted for 11.86%, 17.41%, and 34.86% of the study area, respectively. In 2015, the government directed a reduction of the planting area of spring maize in the \"Liandaowan\" region of Northeast China. The planting area of spring maize was characterized by a continuous increase before this change (2002-2014), exhibited changes and reductions in response to the change (2015-2017), and exhibited optimization and recovery after this change (2018-2020). Compared with the fluctuating and low-frequency planting areas, moderate and severe droughts were higher in stable planting areas. From 2002 to 2020, the most severe droughts occurred in the expanded planting areas. This rapid and large-scale monitoring of spatio-temporal variations and drought of spring maize provides a foundation for improving grain yield. This method could be easily applied to the study of other regions and combined with high-resolution and hyperspectral satellite data to improve monitoring accuracy.
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  • 文章类型: English Abstract
    全球气候变化对人类生产和生活的不利影响日益突出。应对气候变化已成为人类社会面临的严峻挑战,减少温室气体排放已逐渐成为所有国家的共同行动。因此,通过科学方法分析碳排放已成为响应国家“双碳”战略的重要基础。本研究采用省级碳排放统计数据,结合夜间光照数据和人口数据,并将碳排放分配到网格尺度。分析了2000年、2005年、2010年、2015年和2018年中国碳排放的时空特征和演变特征,以及碳排放与经济的相关性。结果表明:①2000-2018年,我国CO2排放总量持续增长,但随着时间的推移,增长率放缓。碳排放的年均增长率从2000-2010年的9.9%下降到2010-2018年的7.4%。从空间分布的角度来看,无碳地区主要分布在西北无人区和东北森林和山区,低碳排放主要分布在广大中小城市和城镇,高碳排放集中在北方,中央,东部沿海,西部省会城市和城市群。②地级市碳排放具有高价值或低价值的集聚;这种集聚总体上趋于稳定,并在2005年后有所增强。低-低集聚区主要分布在西部连片地区和海南岛。随着经济社会的发展,低-低集聚区开始分化,规模缩小;高-高集聚区主要分布在京津冀城市群,太原城市群,长三角城市群,和珠江三角洲城市群,规模逐步加强和巩固;高低高集聚区主要出现在经济发展水平差异较大的周边城市。③中国大部分地区的碳排放相对稳定。碳排放发生变化的地区主要分布在省会和重点城市的周边地区,中心城区无变化,周边地区碳排放量无变化的圆形结构。④从2000年到2018年,中国城市发展的总体过程经历了从“低排放-低收入”到“高排放-低收入”到“高排放-高收入”,最后到“低排放-高收入”的转变。“中国的碳排放增长速度正在放缓。在"双碳"战略的背景下,由于碳排放状况的不同,不同地区面临着不同的碳减排任务和压力。因此,区分碳排放政策应按地区和行业实施。
    The adverse effects of global climate change on human production and life are becoming increasingly prominent. Responding to climate change has become a severe challenge faced by human society, and the reduction in greenhouse gas emissions has gradually become a common action by all countries. Therefore, analyzing carbon emissions through scientific methods has become an important foundation for responding to the national \"dual carbon\" strategy. This study used provincial-level carbon emission statistics, combined with nighttime light data and population data, and assigned carbon emissions to the grid scale. It also analyzed the temporal and spatial characteristics and evolution characteristics of carbon emissions in China in 2000, 2005, 2010, 2015, and 2018, as well as the correlation between carbon emissions and the economy. The results showed that:① from 2000 to 2018, the total CO2 emissions in China continued to grow, but the growth rate slowed over time. The average annual growth rate of carbon emissions dropped from 9.9% in 2000-2010 to 7.4% in 2010-2018. From the perspective of spatial distribution, carbon-free areas were mainly distributed in the northwest uninhabited area and northeast forest and mountainous areas, low-carbon emissions were mainly distributed in the vast small and medium-sized cities and towns, and high-carbon emissions were concentrated in northern, central, eastern coastal, and western provincial capitals and urban agglomerations. ② Carbon emissions had high-value or low-value agglomerations at prefecture-level cities; this agglomeration tended to stabilize as a whole and had strengthened after 2005. Low-low agglomeration areas were mainly distributed in the western contiguous areas and Hainan Island. With economic and social development, low-low agglomeration areas began to fragment and reduce in size; high-high agglomeration areas were mainly distributed in the Beijing-Tianjin-Hebei urban agglomeration, Taiyuan urban agglomeration, Yangtze River Delta urban agglomerations, and Pearl River Delta urban agglomerations, and the scale was gradually strengthened and consolidated; high-low and low-high agglomeration areas mainly appeared in neighboring cities with large differences in economic development levels. ③ Carbon emissions in most parts of China were relatively stable. The areas where carbon emissions had changed were mainly distributed in the peripheral areas of provincial capitals and key cities, and there was a circle structure with no changes in the central urban area and changes in carbon emissions in the peripheral areas. ④ The overall process of urban development in China from 2000 to 2018 followed a shift from \"low emission-low income\" to \"high emission-low income\" to \"high emission-high income\" and finally to \"low emission-high income.\" The growth rate of carbon emissions in China is slowing down. Under the background of the \"dual carbon\" strategy, different regions face different carbon emission reduction tasks and pressures due to different carbon emission situations. Therefore, the differentiated carbon emissions policy should be implemented by regions and industries.
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  • 文章类型: Journal Article
    多环芳烃(PAHs)和重金属(HM)是持续存在的环境问题。二次排放是由于气候变化和人类活动而产生的。为了观察PAHs和HMs的时空变化,并讨论沉积物和泥炭中PAHs的来源以及来源或汇,在大九湖地区沿流向井下的方向选择了12个地表沉积物和地表水点,同时,在泥炭地收集了表面泥炭和水样。连续取样三年(9月。2018年9月2019年和9月分别于2020年)。结果表明,多环芳烃和HMs在沉积物和泥炭中普遍存在。泥炭和水中的PAHs浓度通常较高,虽然HMs在水中的浓度相对较高,在沉积物和泥炭中的浓度相对较低,沉积物的生态风险较低。沉积物中的HMs主要受岩石风化影响,虽然多环芳烃主要受大气沉降影响,生物质和煤炭燃烧和车辆排放。HMs和PAHs可以作为大九湖地区岩石风化和人类活动的指标,分别。水-沉积物逸度分析表明,泥炭是PAHs的水槽,确认它具有很高的吸附有机污染物的能力,沉积物是PAHs的次要来源,可以将它们释放到水中。应注意泥炭地逸度分数(ff)值的增加,表明泥炭可能从汇转化为PAHs来源。
    Polycyclic aromatic hydrocarbons (PAHs) and heavy metals (HMs) are persistent environmental issues. Secondary emissions are produced as a result of climate change and human activity. To observe spatio-temporal variations of PAHs and HMs and to discuss the sources as well as the source or sink of PAHs for sediment and peat, twelve surface sediment and surface water sites were chosen along the direction of the flow to down hole in the Dajiuhu area, simultaneously, surface peat and water samples were collected in peatland. Samples were continuously taken for three years (Sep. 2018, Sep. 2019, and Sep. 2020, respectively). The results showed that PAHs and HMs are common in sediment and peat. PAHs concentration is generally higher in peat and water, while HMs concentration is relatively higher in water and relatively low in sediment and peat, and the ecological risk of sediment was low. HMs in sediment are mainly affected by rock weathering, while PAHs are mainly affected by atmospheric deposition, biomass and coal combustion and vehicle emission. HMs and PAHs can be used as an indicator of rock weathering and human activity in Dajiuhu area, respectively. A water-sediment fugacity analysis revealed that peat is a sink for PAHs, confirming that it has a high capacity for adsorbing organic contaminants, and that sediments are secondary sources of PAHs that can release them into water. Attention should be paid to the increased fugacity fraction (ff) value in peatland, indicating that peat might be converted from a sink to a source of PAHs.
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