Greenhouse gas

温室气体
  • 文章类型: Journal Article
    在城市一级推动温室气体(GHG)和空气污染物(AP)的共同减排对于促进社会绿色和低碳转型至关重要。然而,这一层面的全面和精细研究仍然有限。为了促进城市对温室气体控制和减少AP的精细管理,本研究针对上海九类人为排放源,一个典型的中国大城市,分析三种类型的温室气体(CO2、CH4、N2O)和七种类型的AP(SO2、NOx、CO,VOCs,NH3、PM2.5、PM10)通过排放流,空间分布,热点区域识别,和情景预测。结果强调了不同类型的来源异质性和能源消耗的显着贡献。CO2排放与SO2、NOx、CO,其次是VOCs和PM。CO2-VOCs的热点地区,CO2-NOx和CO2-SO2共同减排包括发电厂,南部沿海地区的石化企业和化工园区,北部沿海地区的钢铁企业和发电厂,中部和东部沿海地区的机场地区,提供了巨大的潜在最大的减少好处。在工业部门实现积极的共同利益将取决于发电和钢铁行业二氧化碳排放量的稳步下降。引入碳捕获装置和提高能源效率将更有利于减少二氧化碳排放,在增加清洁能源份额和逐步淘汰过时车辆的同时,机械,或生产能力在减少AP方面更有效。到2050年,这些缓解措施可以分别减少68.8%和47.6%的二氧化碳排放量。随着这些措施的不断实施,CO2和AP减排的共同作用将逐渐增强。
    Driving co-abatement of Greenhouse Gas (GHGs) and Air Pollutants (APs) in the city level is crucial for fostering societal green and low-carbon transitions, yet comprehensive and refined researches at this level remain limited. To facilitate urban fine management of GHGs control and APs reduction, this study targeted nine categories of anthropogenic emission sources in Shanghai, a typical megacity of China, analyzing the co-benefits of three types of GHGs (CO2, CH4, N2O) and seven types of APs (SO2, NOx, CO, VOCs, NH3, PM2.5, PM10) via emissions flow, spatial distribution, hotspot regions identification, and scenario prediction. Results highlighted the source heterogeneity of different types and significant contributions of energy consumption. CO2 emissions showed a strong spatial correlation with SO2, NOx, and CO, followed by VOCs and PM. Hotspot regions for CO2-VOCs, CO2-NOx and CO2-SO2 co-abatement included power plants, petrochemical enterprises and chemical industrial parks in the southern coastal areas, iron and steel enterprises and power plants in the northern coastal areas, and airport areas in the central and eastern coastal areas, presenting great potential maximum reduction benefits. Achieving positive co-benefits in industrial sector would depend on the steady decline of CO2 emissions in power generation and steel industries. Introducing carbon capture devices and improving energy efficiency would be more beneficial to CO2 emission reduction, while increasing the share of clean energy and phasing out outdated vehicles, machinery, or production capacities are more effective in reducing APs. These mitigation measures could achieve 68.8 % and 47.6 % reduction for CO2 and APs by 2050, respectively, and the co-effect of CO2 and APs emission reduction would gradually increase with the continuous implementation of these measures.
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  • 文章类型: Journal Article
    背景:上天生物圈和局部排放的温室气体观测(GOBLEU)是日本宇宙航空研究开发机构(JAXA)和ANAHOLDINGINC的新联合项目。(ANAHD),运营ANA航班。GOBLEU旨在通过收集温室气体(GHG)数据以及相关排放数据(二氧化亚氮,NO2)和去除(太阳诱导荧光,SIF)来自定期客运航班。我们基于JAXA为日本温室气体观测卫星(GOSAT)开发的空间遥感技术开发了一种行李大小的仪器。该仪器可以方便地安装在教练级乘客座椅上,而无需修改座椅或飞机。
    结果:在从东京羽田机场飞往福冈机场的航班上进行了首次GOBLEU观测,只有NO2模块被激活。将收集到的高空间分辨率NO2数据与来自TROPOMI卫星的数据和来自地面空气质量监测站的地面NO2数据进行了比较。虽然GOBLEU和TROPOMI数据分享了主要由城市和大型点源驱动的主要集中模式,不管不同的观察时间,我们发现了精细尺度的浓度模式差异,这可能表明GOBLEU有可能带来新的排放信息,因此值得进一步研究。我们还表征了随时间变化的NO2空间相关性水平。GOBLEU和TROPOMI的相关性水平迅速下降表明,CO2和NO2之间的时间差作为排放标记物可能会产生重大影响,因此,未来太空任务计划的同一地点观测的重要性。
    结论:GOBLEU提出了基于飞机的,成本效益高,定期客机上携带的GOBLEU仪器经常监测温室气体排放。理论上,GOBLEU仪器可以在大多数商业使用的客机上安装和操作,而无需修改。JAXA和ANAHD希望通过加强《巴黎协定》下的国际合作,将观测范围和伙伴关系扩大到其他国家,从而促进观测技术。
    BACKGROUND: The Greenhouse gas Observations of Biospheric and Local Emissions from the Upper sky (GOBLEU) is a new joint project by Japan Aerospace Exploration Agency (JAXA) and ANA HOLDING INC. (ANAHD), which operates ANA flights. GOBLEU aims to visualizes our climate mitigation effort progress in support of subnational climate mitigation by collecting greenhouse gas (GHG) data as well as relevant data for emissions (nitrous dioxide, NO2) and removals (Solar-Induced Fluorescence, SIF) from regular passenger flights. We developed a luggage-sized instrument based on the space remote-sensing techniques that JAXA has developed for Japan\'s Greenhouse gas Observing SATellite (GOSAT). The instrument can be conveniently installed on a coach-class passenger seat without modifying the seat or the aircraft.
    RESULTS: The first GOBLEU observation was made on the flight from the Tokyo Haneda Airport to the Fukuoka Airport, with only the NO2 module activated. The collected high-spatial-resolution NO2 data were compared to that from the TROPOspheric Monitoring Instrument (TROPOMI) satellite and surface NO2 data from ground-based air quality monitoring stations. While GOBLEU and TROPOMI data shared the major concentration patterns largely driven by cities and large point sources, regardless of different observation times, we found fine-scale concentration pattern differences, which might be an indication of potential room for GOBLEU to bring in new emission information and thus is worth further examination. We also characterized the levels of NO2 spatial correlation that change over time. The quickly degrading correlation level of GOBLEU and TROPOMI suggests a potentially significant impact of the time difference between CO2 and NO2 as an emission marker and, thus, the significance of co-located observations planned by future space missions.
    CONCLUSIONS: GOBLEU proposes aircraft-based, cost-effective, frequent monitoring of greenhouse emissions by GOBLEU instruments carried on regular passenger aircraft. Theoretically, the GOBLEU instrument can be installed and operated in most commercially used passenger aircraft without modifications. JAXA and ANAHD wish to promote the observation technique by expanding the observation coverage and partnership to other countries by enhancing international cooperation under the Paris Agreement.
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  • 文章类型: Journal Article
    目的:研究已经证明了面对面会议对环境的负面影响。尽管如此,面对面会议有好处。2023年美国小儿外科协会(APSA)会议大多是亲自参加的。为了了解对环境的影响,这项研究量化了那次会议产生的旅行排放。
    方法:2023年APSA会议在奥兰多举行,FL.使用取消标识的与会者列表,与会者的家乡城市和奥兰多之间的距离已经确定。如果≤200英里,假设与会者开车。如果超过200英里,确定了最近的机场和奥兰多国际机场之间的距离。旅行排放因子表示每人英里旅行的排放量。环境保护局(EPA)温室气体清单二氧化碳(CO2)的排放因子,甲烷(CH4),和一氧化二氮(N2O)乘以旅行距离,以确定每个与会者产生的排放量。将这些汇总以确定会议旅行的总排放量。EPA温室气体当量计算器用于将排放量转换为相关结果。
    结果:有757名现场参与者和135名虚拟参与者。50名与会者开车,707名与会者乘飞机。这产生了267,279千克二氧化碳,1222克CH4和8486克N2O;相当于美国每年平均使用60辆汽油动力乘用车产生的排放量。
    结论:根据参加2023年APSA会议的情况,最好是亲自见面,尽管相关的环境成本应该得到承认。基于这些结果,APSA应考虑减轻其年度会议对环境的影响的战略。
    方法:不适用。
    OBJECTIVE: Research has demonstrated negative environmental impacts from in-person conferences. Nonetheless, there are benefits to in-person meetings. The 2023 American Pediatric Surgical Association (APSA) meeting was mostly attended in-person. To understand the environmental impact, this study quantifies the travel emissions generated from that meeting.
    METHODS: The 2023 APSA meeting was held in Orlando, FL. Using a de-identified list of attendees, the distance between the attendee\'s home city and Orlando was determined. If ≤ 200 miles, it was assumed the attendee drove. If > 200 miles, the distance between the closest airport and Orlando International Airport was determined. Travel emissions factors represent emissions per person-mile traveled. The Environmental Protection Agency (EPA) Greenhouse Gas Inventory emissions factors for carbon dioxide (CO2), methane (CH4), and nitrous oxide (N2O) were multiplied by travel distances to determine the emissions generated from each attendee. These were aggregated to determine the total meeting travel emissions. The EPA Greenhouse Gas Equivalencies Calculator was used to convert the emissions to a relatable outcome.
    RESULTS: There were 757 in-person and 135 virtual attendees. Fifty attendees drove and 707 attendees flew. This generated 267,279 kg CO2, 1222 gm CH4, and 8486 gm N2O; equivalent to the emissions generated from the average annual use of 60 gasoline-powered passenger vehicles in the United States.
    CONCLUSIONS: Based on attendance to the 2023 APSA meeting, there is a preference for meeting in-person, though the associated environmental cost should be recognized. Based on these results, APSA should consider strategies to mitigate the environmental impact of its annual meeting.
    METHODS: N/A.
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  • 文章类型: Journal Article
    该研究旨在研究补充禽源多克隆抗体(PAP)对瘤胃产甲烷菌甲烷菌(PAP-Ho)和反刍动物M1(PAP-M1)对安格斯杂交牛瘤胃发酵状况和甲烷产生的影响牛(13头和1头母牛)。实验采用3×2+1阶乘排列的随机区组设计,在三个时期复制。因素包括混合物中PAP与Ho和M1的比例(100:0、50:50和0:100Ho:M1)和每种混合物的水平(每d3-或6-mL)。对照治疗中的牛没有接受PAP补充。在处理的第0、14和21天从动物中收集瘤胃液以确定瘤胃发酵曲线和离体甲烷产生。包合水平对离体甲烷产生没有影响。补充PAP-M1,单独或与PAP-Ho联合使用,与对照组相比,离体甲烷输出量降低。此外,单独使用PAP-M1或与PAP-Ho联合使用时,丙酸盐的体内摩尔比例趋于更大,与对照组相比。该研究得出结论,针对瘤胃产甲烷菌的多克隆抗体具有减少牛肠甲烷排放的潜力。该研究为PAP作为减少牛温室气体排放的策略的潜在用途提供了重要见解。需要进一步的研究来证实这些发现,并确定使用PAP的实用性和可行性。
    The study aimed to investigate the effect of supplementing polyclonal antibodies (PAP) of avian origin against the ruminal methanogens Methanobrevibacter gottschalkii Ho (PAP-Ho) and M. ruminantium M1 (PAP-M1) on ruminal fermentation profile and methane production in Angus crossbred cattle (13 steers and 1 heifer). The experiment was conducted using a randomized block design with a 3 × 2 + 1 factorial arrangement, replicated in three periods. The factors included proportions of PAP against Ho and M1 in the mixture (100:0, 50:50, and 0:100 Ho:M1) and level of each mixture (3- or 6-mL per d). Cattle in control treatment did not receive PAP supplementation. Ruminal fluid was collected from the animals on d 0, 14 and 21 of treatment to determine of ruminal fermentation profile and ex vivo methane production. There was no effect of level of inclusion on ex vivo methane production. Supplementation with PAP-M1, either alone or in combination with PAP-Ho, decreased ex vivo methane output compared to the control group. Furthermore, in vivo molar proportion of propionate tended to be greater with PAP-M1, alone or combined with PAP-Ho, when compared with the control group. The study concluded that polyclonal antibodies against ruminal methanogens have the potential to decrease enteric methane emissions in cattle. The research provided important insights into the potential use of PAP as a strategy for reducing greenhouse gas emissions from cattle. Further research is needed to confirm these findings and to determine the practicality and feasibility of using PAP.
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  • 文章类型: Journal Article
    气候变化和环境污染对健康有已知影响。美国政府最近出台的降低通胀法案(IRA)包括遏制气候变化的资助举措,减少环境污染,根据国家自主贡献(NDC)计划(与2005年相比,到2030年温室气体[GHG]排放量减少40-50%)。目前尚不清楚IRA驱动的气候行动对实现NDC目标的预期心血管健康益处。
    我们使用了能源政策模拟器(EPS),一种基于系统动力学建模的模拟算法,估计各种能源政策的影响,模拟到2050年在美国实现NDC目标对健康结果的影响。我们进一步调查了到2050年种族对死亡率(绝对和相对)的影响。我们估计2022年至2050年之间的6种不良健康结果的预计减少:哮喘发作,非致命性心脏病发作,入院,呼吸道症状和支气管炎,丢失的工作日,和死亡。
    到2050年实现NDC目标将导致987,415避免哮喘发作,41,565避免了非致命性心脏病发作,18,993避免了入院,1,493,010避免了呼吸道症状和支气管炎,3,317,250避免了工作日的损失,和32,659人避免了死亡(22,839人在白人中,4993个黑人个体,2801亚洲人,和2026年其他/多种族个体)。到2050年,少数族裔群体在避免死亡方面有更高的相对变化(白人-0.74%,黑色-1.01%,亚洲-1.24%,和其他/多种族-1.75%)。同样,到2050年,与非西班牙裔/拉丁美洲人(-0.7%)相比,西班牙裔/拉丁美洲人的死亡人数相对减少(-1.4%)。
    IRA促进到2050年实现NDC温室气体减排目标将导致大量避免不良健康结果和死亡。预计到2050年,种族和少数民族的死亡人数相对减少幅度最大。本报告强调了无论政治分歧如何,持续进行气候行动投资的重要性。IRA这方面的认识可能对整体健康保护更为重要,除了降低药物成本。
    UNASSIGNED: Climate change and environmental pollution have known health effects. The recently introduced inflation reduction act (IRA) by the United States government includes funding initiatives to curb climate change, and reduce environmental pollution, in line with the nationally determined contribution (NDC) plan (40-50 % reduction in greenhouse gas [GHG] emissions by 2030, as compared with 2005). The projected cardiovascular health benefits of the IRA driven climate actions to achieve the NDC goals are not known.
    UNASSIGNED: We used the Energy Policy Simulator (EPS), a simulation algorithm based on systems dynamics modelling estimating the impact of various energy policies, to model the impact of achieving NDC targets in the United States on health outcomes by 2050. We further investigated race-specific impact on mortality (absolute and relative) by 2050.We estimated the projected reduction in six adverse health outcomes between 2022 and 2050: asthma attacks, non-fatal heart attacks, hospital admissions, respiratory symptoms and bronchitis, lost workdays, and deaths.
    UNASSIGNED: Achievement of NDC targets by 2050 will result in 987,415 avoided asthma attacks, 41,565 avoided nonfatal heart attacks, 18,993 avoided hospital admissions, 1,493,010 avoided respiratory symptoms and bronchitis, 3,317,250 avoided lost workdays, and 32,659 avoided deaths (22,839 among white individuals, 4993 among Black individuals, 2801 among Asian individuals, and 2026 among other/multirace individuals). By 2050, minority racial groups had higher relative change in avoided deaths (white -0.74 %, Black -1.01 %, Asian -1.24 %, and other/multirace -1.75 %). Similarly, Hispanics/latinos higher relative reductions in deaths (-1.4 %) compared with non-Hispanic/Latinos (-0.7 %) by 2050.
    UNASSIGNED: The IRA facilitated achievement of NDC GHG reduction goals by 2050 would result in substantial number of avoided adverse health outcomes and death. Racial and ethnic minorities are expected to have the largest relative reductions in deaths by 2050. The current report underscores the importance of continued climate action investment irrespective of political differences. The appreciation of this aspect of the IRA may be more important to overall preservation of health, beyond the reduction in medication costs.
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  • 文章类型: Journal Article
    中国沿海的盐沼受到互花米草入侵的威胁(S.互花米草)。这项研究是在安东浅滩进行的,杭州湾,中国,目的是了解互花米草入侵对温室气体(GHG)生产和排放的复杂影响。为了解决这个问题,我们彻底检查了溶解有机物(DOM)的化学性质和地表水-孔隙水相互作用的速率。从农田收集了前水和地表水样本,互花米草入侵地区,和Scirpusmarqueter(S.marqueter)主导地区。研究结果表明,互花米草的入侵阻碍了地表水与孔隙水的相互作用,导致其受影响区域内的孔隙水交换率降低(0.015-0.440cmd-1),与大麻素占主导地位的地区(9.635-18.232cmd-1)相反。入侵还增加了孔隙水中溶解的有机碳浓度,并创造了一个稳定而封闭的土壤环境,导致DOM具有较小的分子大小和较高的腐殖水平。高色氨酸样荧光DOM的存在导致互花米草入侵地区甲烷和二氧化碳的产生增加。然而,有限的表面-孔隙水交换以及孔隙水和地表水之间温室气体浓度的显着差异表明,互花米草的通生组织可能在将温室气体从土壤输送到大气中起重要作用。
    Saltmarshes along the Chinese coast are threatened by the invasion of Spartina alterniflora (S. alterniflora). This study was carried out in the Andong Shoal, Hangzhou Bay, China, with the aim of comprehending the intricate impacts of S. alterniflora invasion on greenhouse gases (GHG) production and emissions. To address this issue, we thoroughly examined the chemistry of dissolved organic matter (DOM) and the rate of surface water-porewater interaction. Porewater and surface water samples were collected from farm land, S. alterniflora invaded areas, and Scirpus mariqueter (S. mariqueter) dominated areas. The findings indicated that the invasion of S. alterniflora impeded the interaction between surface water and porewater, resulting in reduced porewater exchange rates within its affected region (0.015-0.440 cm d-1), in contrast to areas dominated by S. mariqueter (9.635-18.232 cm d-1). The invasion also increased dissolved organic carbon concentration in porewater and created a stable and closed soil environment that resulted in DOM with smaller molecule sizes and higher humification levels. The presence of high tryptophan-like fluorescent DOM caused an increase in the production of methane and carbon dioxide in S. alterniflora invaded area. However, both limited surface-porewater exchange and significant differences in GHG concentrations between porewater and surface water suggested that the aerenchyma tissues of S. alterniflora may play an important role in transporting GHG from soil to the atmosphere.
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  • 文章类型: Journal Article
    人工湿地(CWs)中的低效脱氮可归因于低碳氮比(C/N)废水的碳源不足。在这项研究中,以甘蔗渣发酵液(SBFL)为补充碳源,在间歇曝气的CW中增强脱氮能力。研究了不同调节进水C/N比对脱氮和温室气体(GHG)排放的影响。结果表明,SBFL的添加显著提高了反硝化能力,与蔗糖相比,NO3--N的去除速度更快。此外,与非充气CW相比,间歇充气CW显着提高了NH4-N的去除效率。在添加SBFL的间歇曝气CW中,进水C/N比为5时,总氮去除效率最高(98.3%)。与蔗糖相比,SBFL的添加导致N2O排放减少17.8%-43.7%。所有CW都显示出低CH4排放,与蔗糖相比,添加SBFL(0.035-0.066mg·m-2h-1)的排放量较低。此外,反硝化的丰度较高(NirK,在SBFL输入的CW中显示了nirS和nosZ)基因以及更丰富的反硝化细菌。本研究结果为应用SBFL作为碳源提高CW的脱氮效率和减少GHG排放提供了可行的策略。
    The inefficient nitrogen removal in constructed wetlands (CWs) can be attributed to insufficient carbon sources for low carbon-to-nitrogen (C/N) ratio wastewater. In this study, sugarcane bagasse fermentation liquid (SBFL) was used as a supplemental carbon source in intermittently aerated CWs to enhance nitrogen removal. The impact of different regulated influent C/N ratios on nitrogen removal and greenhouse gas (GHG) emissions was investigated. Results demonstrated that SBFL addition significantly enhanced the denitrification capacity, resulting in faster NO3--N removal compared to sucrose. Moreover, intermittently aerated CWs significantly improved NH4+-N removal efficiency compared to non-aerated CWs. The highest total nitrogen removal efficiency (98.3 %) was achieved at an influent C/N ratio of 5 in intermittently aerated CWs with SBFL addition. The addition of SBFL resulted in a reduction of N2O emissions by 17.8 %-43.7 % compared to sucrose. All CWs exhibited low CH4 emissions, with SBFL addition (0.035-0.066 mg·m-2h-1) resulting in lower emissions compared to sucrose. Additionally, higher abundance of denitrification (nirK, nirS and nosZ) genes as well as more abundant denitrifying bacteria were shown in CWs of SBFL inputs. The results of this study provide a feasible strategy for applying SBFL as a carbon source to improve nitrogen removal efficiency and mitigate GHG emissions in CWs.
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  • 文章类型: Journal Article
    由于再生纸材料的异质性和生产条件,造纸废水中的污染物随时间急剧波动。造纸废水处理工艺(PWTP)的质量控制具有挑战性且成本高昂。随着有关PWTP对温室气体(GHG)排放的环境影响的法规也越来越多,能源消耗,等。,PWTP制定了一个复杂的多目标优化问题。本研究建立了一个多主体深度强化学习框架,以同时优化过程成本,能源消耗,和PWTP中的温室气体排放,根据出水水质,为了实现经济,能源,和环境(3E)目标。使用基准模拟模型No.模拟了造纸厂废水的生物处理过程。1(BSM1)。基于BSM手册生成的数据用于模型训练,并使用从当地造纸厂获得的真实数据来估计模型性能。结果表明,该方法在识别多目标的最佳控制策略方面优于常规技术。
    Due to the heterogeneity of recycled paper materials and the production conditions, pollutants in papermaking wastewater fluctuate sharply over time. Quality control of the papermaking wastewater treatment process (PWTP) is challenging and costly. As regulations are also growing about the environmental effects of the PWTP on greenhouse gas (GHG) emission, energy consumption, etc., the PWTP formulates a complex multiobjective optimization problem. This research established a multiagent deep reinforcement learning framework to simultaneously optimize process cost, energy consumption, and GHG emission in the PWTP, subjected to the effluent quality, to realize economic, energy, and environmental (3E) goals. The biological treatment process of wastewater in paper mills was simulated using benchmark simulation model no. 1 (BSM1). The data generated based on the BSM manual was utilized for model training, and real data acquired from a local papermaking factory was used to estimate the model performance. The results show that the proposed method outperforms conventional techniques in identifying the best control strategies for multiple targets.
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  • 文章类型: Journal Article
    乙烷,在广阔的缺氧环境中第二丰富的气态碳氢化合物,是一种被忽视的温室气体。乙烷的微生物厌氧氧化可以由可用的电子受体如硫酸盐和硝酸盐驱动。然而,尽管亚硝酸盐是比硫酸盐或硝酸盐更热力学可行的电子受体,对亚硝酸盐驱动的厌氧乙烷氧化知之甚少。在这项研究中,通过长期运行亚硝酸盐和乙烷进料生物反应器,富集了能够进行亚硝酸盐驱动的厌氧乙烷氧化的微生物培养物。在连续运行期间,亚硝酸盐去除率和理论乙烷氧化速率分别稳定在约25.0mgNO2-NL-1d-1和11.48mgC2H6L-1d-1。批量测试表明,在这种微生物培养物中,乙烷对于亚硝酸盐的去除至关重要。代谢功能分析显示,与红环菌科中的一个新属有联系的物种,指定为“念珠菌亚硝基还原”,可以进行亚硝酸盐驱动的厌氧乙烷氧化。在提出的代谢模型中,尽管没有已知的基因乙烷转化为乙基琥珀酸和琥珀酸辅酶A连接酶,\'Ca.亚硝基还原菌编码用于厌氧乙烷氧化的预期富马酸盐添加途径和用于亚硝酸盐还原为氮的完全反硝化途径。这些发现促进了我们对亚硝酸盐驱动的厌氧乙烷氧化的理解,强调了先前被忽视的厌氧乙烷氧化对自然生态系统的影响。
    Ethane, the second most abundant gaseous hydrocarbon in vast anoxic environments, is an overlooked greenhouse gas. Microbial anaerobic oxidation of ethane can be driven by available electron acceptors such as sulfate and nitrate. However, despite nitrite being a more thermodynamically feasible electron acceptor than sulfate or nitrate, little is known about nitrite-driven anaerobic ethane oxidation. In this study, a microbial culture capable of nitrite-driven anaerobic ethane oxidation was enriched through the long-term operation of a nitrite-and-ethane-fed bioreactor. During continuous operation, the nitrite removal rate and the theoretical ethane oxidation rate remained stable at approximately 25.0 mg NO2 -N L-1 d-1 and 11.48 mg C2H6 L-1 d-1, respectively. Batch tests demonstrated that ethane is essential for nitrite removal in this microbial culture. Metabolic function analysis revealed that a species affiliated with a novel genus within the family Rhodocyclaceae, designated as \'Candidatus Alkanivoras nitrosoreducens\', may perform the nitrite-driven anaerobic ethane oxidation. In the proposed metabolic model, despite the absence of known genes for ethane conversion to ethyl-succinate and succinate-CoA ligase, \'Ca. A. nitrosoreducens\' encodes a prospective fumarate addition pathway for anaerobic ethane oxidation and a complete denitrification pathway for nitrite reduction to nitrogen. These findings advance our understanding of nitrite-driven anaerobic ethane oxidation, highlighting the previously overlooked impact of anaerobic ethane oxidation in natural ecosystems.
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  • 文章类型: Journal Article
    干旱地区的水库通常提供关键的水存储,但对其温室气体(GHG)足迹知之甚少。虽然人们越来越认识到水库作为温室气体来源的作用,对干旱地区水库的温室气体排放动态及其对环境政策的影响缺乏了解。在这里,我们介绍了鲍威尔湖的初始温室气体排放测量,美国西南部沙漠中的一个大型储水水库。我们报告了水库浅层(<15m)沿海地区的CO2-eq排放量高于水库的全球平均面积排放量(9.4与5.8gCO2-eqm-2d-1),而主要储层的通量低了两个数量级(0.09gCO2-eqm-2d-1)。然后,我们使用四个全球尺度模型将我们的测量结果与储层的CO2CH4排放模型进行了比较。与基于化石燃料的能源相比,将这些排放考虑到鲍威尔湖的水电生产中,每MWh-1的温室气体排放量较低。除了一个模型,TheestimatedhydrocticemissionsforLakePowellrangefrom10-32kgCO2-eqMWh-1,composedto~400-1000kgCO2-eqMWh-1fornaturalgas,油,和煤炭。我们还估计,在低水位下减少沿海栖息地会导致每兆瓦时二氧化碳当量排放量减少50%。温室气体排放对水库水位的敏感性表明,这种相互作用将是干旱地区系统设计和运行中的重要政策考虑因素。
    Reservoirs in arid regions often provide critical water storage but little is known about their greenhouse gas (GHG) footprint. While there is growing appreciation of the role reservoirs play as GHG sources, there is a lack of understanding of GHG emission dynamics from reservoirs in arid regions and implications for environmental policy. Here we present initial GHG emission measurements from Lake Powell, a large water storage reservoir in the desert southwest United States. We report CO2-eq emissions from the shallow (< 15 m) littoral regions of the reservoir that are higher than the global average areal emissions from reservoirs (9.4 vs. 5.8 g CO2-eq m-2 d-1) whereas fluxes from the main reservoir were two orders of magnitude lower (0.09 g CO2-eq m-2 d-1). We then compared our measurements to modeled CO2 + CH4 emissions from the reservoir using four global scale models. Factoring these emissions into hydropower production at Lake Powell yielded low GHG emissions per MWh-1 as compared to fossil-fuel based energy sources. With the exception of one model, the estimated hydropower emissions for Lake Powell ranged from 10-32 kg CO2-eq MWh-1, compared to ∼400-1000 kg CO2-eq MWh-1 for natural gas, oil, and coal. We also estimate that reduced littoral habitat under low water levels leads to ∼50% reduction in the CO2 equivalent emissions per MWh. The sensitivity of GHG emissions to reservoir water levels suggests that the interaction will be an important policy consideration in the design and operation of arid region systems.
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