Environment risk

  • 文章类型: Journal Article
    2018年,中国实施了减少兽用抗菌药物使用行动,以遏制抗生素耐药性(AR)的快速发展。然而,减排政策后动物养殖场与AR相关的污染调查不充分。这里,我们结合UPLC-MS/MS进行了全面的调查,宏基因组,并对广东8个有代表性的大型养鸡场进行了细菌基因组分析,中国。我们的结果表明,肉鸡养殖场的抗生素和ARGs污染比蛋鸡养殖场更严重。值得注意的是,不同的tet(X)变体在养鸡场中普遍存在。这些tet(X)由不同的大肠杆菌谱系携带,并且与ISCR2和IS1B转座酶明显相关。养鸡场的抗性与微生物群落显著相关,多因素分析表明,抗生素-微生物群落-MGEs的联合作用是ARGs的最主要驱动因素。宿主追踪鉴定了多种ARG细菌宿主和ARGs-MRGs-MGE的共存。来源追踪表明,固有成分代表了不同宿主中抗性的主要特征,而鸡肠和农场环境之间的ARG转移很频繁。对AR风险的多视角评估表明,减少抗生素的早期效果是通过减轻最大水平的风险ARGs来表现的。环境AR病原体的流行,和由噬菌体结构介导的ARGs的HGT潜力。总的来说,我们的研究结果为不同饲养策略的大型养鸡场的抗生素和ARG概况提供了见解,并初步展示了中国减少抗生素行动的表现。
    In 2018, China implemented the Veterinary Antimicrobial Use Reduction Action to curb the rapid development of antibiotic resistance (AR). However, the AR-related pollutions in animal farms after the reduction policy has been poorly investigated. Here, we performed a comprehensive investigation combining UPLC-MS/MS, metagenomic, and bacterial genomic analyses in eight representative large-scale chicken farms in Guangdong, China. Our results showed that antibiotics and ARGs contaminations were more severe in broiler farms than in layer farms. Notably, diverse tet(X) variants were prevalent in the chicken farms. These tet(X)s was carried by diverse E. coli lineages and obviously correlated with ISCR2 and IS1B transposases. The resistomes in chicken farms was significantly correlated with microbial community, and multiple factor analyses indicated that the joint effect of antibiotics-microbial community-MGEs was the most dominant driver of ARGs. Host tracking identified a variety of ARG bacterial hosts and the co-occurrence of ARGs-MRGs-MGEs. Source tracking indicated that the inherent component represented the main feature of resistomes in different hosts, while ARG transfer between the chicken gut and farm environments were frequent. A multiperspective evaluation of AR risk revealed that the early effect of antibiotic reduction was exhibited by the mitigation of maximum level of risky ARGs, prevalence of environmental AR pathogens, and HGT potential of ARGs mediated by phage structures. Overall, our findings provide insights into the antibiotic and ARG profiles in large-scale chicken farms with different rearing strategies and demonstrate a preliminary view of the performance of antibiotic reduction actions in China.
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  • 文章类型: Journal Article
    土壤中的重金属构成严重的生态和健康风险。为了制定有效的策略来减轻潜在的危险,揭示污染源及其与风险的联系至关重要。研究人员研究了土壤中重金属的来源识别和风险评估,然而,很少有人系统地破译土壤金属的源-汇关系以及源分配和风险评估之间的联系。在研究中,提出了一个综合技术框架来弥补差距,并用于表征污染风险,中国典型煤炭资源城市土壤金属的来源及其联系。利用地球化学工具和生态风险指数进行的评估表明,研究区的土壤受到Cd的污染,Hg,Cr,As和Pb在不同程度上,尤其是,Cd和Hg存在显著的生态风险。两个先进的受体模型(多元曲线分辨率加权交替最小二乘法和多线性引擎2)被比较地应用于分配土壤金属的潜在来源,结果表明,这两个模型已经确定了相似的来源(R2>0.90),包括农业活动,大气沉积和工业排放占35.5%-38.3%,30.3%-35.1%,和26.6%-34.1%,分别。然后,这两个模型的分配结果共同用于使用概率风险评估模型评估环境中金属的特定源健康风险。区域内的风险水平总体可接受或可容忍,相对而言,工业排放对土壤金属对公众的非致癌和致癌风险贡献更大。研究结果将帮助管理者设计有针对性的政策,以降低土壤金属的风险,提出的框架为更好地了解全球其他环境中土壤金属的源-风险关系提供了有用的指南。
    Heavy metals in soils pose serious ecological and health risks. To make efficient strategies for mitigating the underlying hazards, it is critical to reveal the pollution sources and their links with the risks. Researchers have investigated source identification and risk evaluation of heavy metals in soils, yet few have systematically deciphered the source-sink relationship of soil metals and the links between source apportionment and risk assessment. In the study, an integrated technological framework has been proposed to address the gaps, and applied to characterize the pollution risks, sources and their links of soil metals in a typical coal resource city in China. The assessment using geochemical tool and ecological risk index shows the soils in study area are polluted by Cd, Hg, Cr, As and Pb in varied degrees, and particularly, Cd and Hg present significant ecological risk. Two advanced receptor models (multivariate curve resolution-weighted alternating least-squares and multilinear engine 2) are comparatively applied for apportioning the potential sources of soil metals, and the results suggest the two models have identified similar sources (r2 > 0.90), including agricultural activities, atmospheric depositions and industrial discharges with contributions of 35.5 %-38.3 %, 30.3 %-35.1 %, and 26.6 %-34.1 %, respectively. Then, apportionment results of the two models are jointly employed for evaluating the source-specific health risks of metals in the environment using a probabilistic risk assessment model. The risk levels within the area are overall acceptable or tolerable, and relatively, the industrial discharges present higher contribution on the non-carcinogenic and carcinogenic risks of soil metals to public. Findings will help the managers to design targeted policies for reducing the risks of soil metals, and the framework proposed provides a useful guideline to better understand the source-risk relationship of soil metals in other environments worldwide.
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  • 文章类型: Journal Article
    热解是处理废弃矿山中植物修复残留物的有效方法,产生有价值的副产品,生物炭。然而,来自这些残留物的生物炭的环境应用受到重金属潜在环境风险的限制。在这里,Miscanthussp.废弃矿山的残留物在不同的热解温度(300-700°C)下热解为生物炭,以促进植物修复残留物的安全再利用。结果表明,热解能显著稳定生物质中的重金属,其中Cd表现出最显著的稳定作用。Cd的酸溶/可交换和可还原部分从69.91%显著下降到2.52%,在700°C时,可氧化和残留部分增加了约3.24倍。环境风险评估表明,超过500°C热解的生物炭具有较低的环境风险(RI<30),使它们成为植物修复残留物安全利用的最佳选择。此外,吸附实验表明,在较高温度(500-700°C)下制备的生物炭表现出优异的吸附能力,归因于碱度和沉淀效应。这项研究强调了热解芒草产生的生物炭。从500°C以上的废弃矿山开始,有望实现环境修复,为富含金属的生物质的再利用提供了新的见解。
    Pyrolysis stands out as an effective method for the disposal of phytoremediation residues in abandoned mines, yielding a valuable by-product, biochar. However, the environmental application of biochar derived from such residues is limited by the potential environmental risks of heavy metals. Herein, Miscanthus sp. residues from abandoned mines were pyrolyzed into biochars at varied pyrolysis temperatures (300-700 °C) to facilitate the safe reuse of phytoremediation residues. The results showed that pyrolysis significantly stabilizes heavy metals in biomass, with Cd exhibiting the most notable stabilization effect. Acid-soluble/exchangeable and reducible fractions of Cd decreased significantly from 69.91 % to 2.52 %, and oxidizable and residue fractions increased approximately 3.24 times at 700 °C. The environmental risk assessment indicated that biochar pyrolyzed over 500 °C pose lower environmental risk (RI < 30), making them optimal for the safe utilization of phytoremediation residues. Additionally, adsorption experiments suggested that biochars prepared at higher temperature (500-700 °C) exhibit superior adsorption capacity, attributed to alkalinity and precipitation effect. This study highlights that biochars produced by pyrolyzing Miscanthus sp. from abandoned mines above 500 °C hold promise for environmental remediation, offering novel insight into the reutilization of metal-rich biomass.
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  • 文章类型: Journal Article
    碳:氮:磷(C:N:P)化学计量在调节农业生态系统中磷的转化中起着至关重要的作用。然而,平衡C:N:P化学计量对水稻土的影响,特别是关于相对土壤磷转化,仍然未知。本研究探讨了C:N:P化学计量对粪肥替代的响应及其在土壤磷转化中的调节作用,以及对环境的相关释放风险。根据一项为期5年的实地研究,我们的发现表明,用猪粪代替30%的化学磷肥(与化学磷肥处理相同的NPK总量,命名为CFM)增加了土壤总碳,而不改变土壤总磷,导致土壤C:P比升高,尽管作物化学计量的稳态。这种增加促进了土壤中微生物的多样性和有机磷的积累。变形菌和放线菌一起产生较低的C:PEEA代谢,并提高了P的体内周转率。此外,通过整合高分辨率透析(HR-Peeper),薄膜中的扩散梯度(DGT),DGT诱导的土壤通量(DIFS),和沉积物磷释放风险指数(SPRRI)模型,我们观察到,除了有机P,CFM同时增加土壤AlP,从而削弱了P从土壤固体向溶液的扩散和再供应能力。因此,P对环境的释放风险有所降低.总的来说,这项研究建立了作物-土壤-酶C:N:P化学计量之间的联系,土壤微生物,和土壤磷的生物地球化学过程。该研究进一步评估了P释放对环境的风险,为粪肥替代对土壤磷循环的直接和间接影响提供了新的视角。
    Carbon:nitrogen:phosphorus (C:N:P) stoichiometry plays a vital role in regulating P transformation in agriculture ecosystems. However, the impact of balanced C:N:P stoichiometry in paddy soil, particularly regarding relative soil P transformation, remains unknown. This study explores the response of C:N:P stoichiometry to manure substitution and its regulatory role in soil P transformation, along with the associated release risk to the environment. Based on a 5-year field study, our findings reveal that replacing 30 % of chemical P fertilizer with pig manure (equal total NPK amounts with chemical P fertilizer treatment, named CFM) increased soil total C without altering soil total P, resulting in an elevated soil C:P ratio, despite the homeostasis of crop stoichiometry. This increase promoted microbial diversity and the accumulation of organic P in the soil. The Proteobacteria and Actinobacteria produced lower C:PEEA metabolism together, and enhanced in vivo turnover of P. Additionally, by integrating high-resolution dialysis (HR-Peeper), diffusive gradients in thin films (DGT), DGT-induced fluxes in the soil (DIFS), and sediment P release risk index (SPRRI) models, we observed that, in addition to organic P, CFM simultaneously increased soil Al-P, thereby weakening the diffusion and resupply capacity of P from soil solids to the solution. Consequently, this decrease in P release risk to the environment was demonstrated. Overall, this study establishes a connection between crop-soil-enzyme C:N:P stoichiometry, soil microorganisms, and soil P biogeochemical processes. The study further evaluates the P release risk to the environment, providing a novel perspective on both the direct and indirect effects of manure substitution on soil P cycling.
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  • 文章类型: Journal Article
    为了应对COVID-19全球大流行带来的经济和社会危害,许多国家已经采用各种信息技术来快速跟踪和控制流行病的传播。健康快速反应码(QR)是中国政府在疫情环境中实施的应急措施,旨在平衡疫情防控与经济和社会发展的恢复。并促进跨区域的公共流动和进入各种公共空间。公众使用健康守则是现实的需要,但是它们的使用满意度受到多种因素的影响,例如环境,技术,和组织。在本文中,通过问卷调查收集数据,分析我国公众对健康二维码使用满意度的基本情况及其影响因素。结果表明,感知质量和平台信任直接影响健康代码使用的满意度,而环境风险和平台信任通过感知质量的中介作用间接影响健康代码使用的满意度。
    In response to the economic and social hazards posed by the COVID-19 global pandemic, many countries have adopted various information technologies to rapidly track and control the spread of the epidemic. Health Quick Response (QR) codes are emergency measures implemented by the Chinese government in the epidemic environment to balance epidemic prevention and control with recovery of economic and social development, and facilitate public mobility across regions and access to various public spaces. The use of health codes by the public is a practical necessity, but the satisfaction of their use is influenced by multiple factors such as environment, technology, and organization. In this paper, we collected data through a questionnaire to analyze the basic situation of public satisfaction with the use of health QR codes in China and its influencing factors. The results show that perceived quality and platform trust directly affect the satisfaction of health code usage, while environmental risk and platform trust indirectly affect the satisfaction of health code usage through the mediating effect of perceived quality.
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  • 文章类型: Journal Article
    进行这项研究是为了评估蔡道和安铜垃圾填埋场在安江省的影响,越南用相对土壤质量指数(RSQI)评价土壤质量潜在生态风险指数(PERI),多变量统计方法和相关的健康风险。分为两层收集了48个土壤样品:A(0-20cm)和B(60-80cm),并分析了雨季和旱季的5个理化土壤参数和8种重金属。结果表明,pH值从弱酸性到中性波动,土壤有机质和养分从贫到中等。重金属浓度在越南标准之内。蔡道垃圾填埋场雨季土壤质量参数的浓度往往较高,但在铜填埋场较低。RSQI在CaiDau和AnCu垃圾填埋场被评为从好到坏,从危险到坏,分别。主成分分析(PCA)和绝对主成分得分-多元线性回归分析证明了垃圾填埋场和农业影响对土壤质量变异性的贡献,占81.38-90.64%。垃圾填埋场对蔡道和安铜的重金属含量贡献了35%和50%以上,分别。CaiDau垃圾填埋场的重金属积累顺序为Ni>Cr>As,但在铜垃圾填埋场没有发现。污染负荷指数(PLI)表明CaiDau和AnCu垃圾填埋场重金属污染的中低风险,分别,因此潜在的生态风险较低。重金属污染土壤的非癌症和癌症风险处于可接受水平。由于其积累特性,需要监测垃圾填埋场周围环境中的重金属。
    The study was conducted to assess the impacts of Cai Dau and An Cu landfills in An Giang province, Vietnam on soil quality using relative soil quality index (RSQI), potential ecological risk index (PERI), and multivariable statistical methods and associated health risks. Forty-eight soil samples were collected in two layers: A (0-20 cm) and B (60-80 cm) and analyzed for five physiochemical soil parameters and eight heavy metals during the rainy and dry seasons. The results showed that pH fluctuated from weak acid to neutral, and organic matters and nutrients in soil were from poor to moderate. Heavy metal concentrations were within the Vietnamese standards. The concentrations of the soil quality parameters tended to be higher during the rainy season at the Cai Dau landfill, but lower at the An Cu landfill. The RSQI was rated as bad to good and hazardous to bad at the Cai Dau and An Cu landfills, respectively. The principal component analysis (PCA) and absolute principal component score-multiple linear regression analysis demonstrated the contribution of landfill and agricultural impacts to soil quality variability, accounting for 81.38-90.64 %. Landfills contributed greater 35 % and 50 % to heavy metal contents at Cai Dau and An Cu, respectively. The heavy metal accumulation at Cai Dau landfill was in the decreasing order of Ni > Cr > As, but that was not found at An Cu landfill. The pollution load index (PLI) indicated medium and low risks of heavy metal contamination at the Cai Dau and An Cu landfills, respectively, thus posing low potential ecological risk. The non-cancer and cancer risks of heavy metals-contaminated soil were at acceptable level. Monitoring of heavy metals in the environments surrounding landfills is needed due to its accumulative characteristics.
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  • 文章类型: Journal Article
    该研究调查了游泳池对医疗保健专业人员从事娱乐活动的意愿的影响,身体焦虑,以及COVID-19背景下的身心健康。本研究采用混合研究方法,用SPSS26.0统计软件检验问卷的信度,然后收集840份有效问卷;首先对数据进行基本统计分析,t检验,方差分析,和PPMCC测试方法,然后采用访谈的方法收集专家意见。多重检查方法汇集了所有数据和讨论。研究发现,采用人员动态跟踪系统或措施,结合次氯酸钠和重复过滤以稳定水质,可以保持大多数医务工作者对游泳池运动环境防疫的信心,避免违规行为。政府可以制定交通安全预防和控制机制,并建立适当的交通路线。接下来,为31-50岁的男性制定了游泳或其他身体活动机制的处方,并为51岁以上的医务人员重新设计了措施,以使他们有紧张的头部问题和身体疲劳,促进血液循环,改善睡眠质量。这将促进医务人员从事游泳运动后缓解压力和调节身心健康的目的。
    The study examined the effects of swimming pools on healthcare professionals\' willingness to engage in recreational activities, physical anxiety, and physical and mental well-being in the context of COVID-19. The research adopted the mixed research method, used SPSS 26.0 statistical software to test the reliability of the questionnaire, and then collected 840 valid questionnaires; first analyzed the data with basic statistics, t-test, ANOVA, and PPMCC test methods, and then used the interview method to collect expert opinions. A multi-check approach assembled all data and discussions. The study found that the use of personnel dynamic tracking systems or measures, combined with sodium hypochlorite and repeated filtration to stabilize water quality, could maintain the confidence of most medical workers in the swimming pool sports environment for epidemic prevention and avoid violations. The government could formulate safety prevention and control mechanisms in traffic and establish appropriate traffic routes. Next, formulated a prescription for swimming or other physical activity mechanisms for men aged 31-50 and redesigned measures for medical staff over 51 years old to have tense head issues and physical fatigue, promote blood circulation and improve sleep quality. This will promote the purpose of relieving stress and regulating the physical and mental health of medical staff after engaging in swimming.
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  • 文章类型: Journal Article
    氟虫腈是一种广泛有效的杀虫剂,属于苯基吡唑化学家族。其作用模式作用于突触前和突触后,通过神经递质GABA阻断氯离子。它被认为是剧毒的,在一些国家,它的使用已被禁止。这篇综述的目的是进行科学计量分析,以对杀虫剂氟虫腈的研究进行全球测量。这项研究中的所有信息都于2021年12月在WebofScience(WoS)数据库中进行了搜索。搜索是使用术语“氟虫腈”进行的。\"因此,选择了2362项研究。大多数选定的文章显示了氟虫腈对非目标生物的毒性作用,检测杀虫剂的分析方法,环境退化过程,以及通过使用减少昆虫的效率。该数据集的H指数为91。作者在国家之间的合作网络显示美国是最臭名昭著的,有30.6%的研究,其次是中国(15.7%)和巴西(10.9%)。关于氟虫腈对蜜蜂的毒性研究很多,退化的形式,和这种杀虫剂的有效性。本工作提出了文章中指出的进一步研究的建议,并强调了涉及氟虫腈的研究的重要性,以及替代害虫控制的研究。
    Fipronil is a broad potent insecticide that belongs to the phenylpyrazole chemical family. Its action mode acting in the presynaptic and postsynaptic blocking the chlorine ions by the neurotransmitters GABA. It is considered highly toxic, and in some countries, its use has been prohibited. The objective of this review is to perform a scientometric analysis for global measurement of the research on the insecticide fipronil. All information in this study was searched in the Web of Science (WoS) database in December 2021. The search was carried using the term \"fipronil.\" Thus, 2362 studies were selected. Most selected articles showed toxicity effects of fipronil on non-target organisms, analytical methods to detect the insecticide, environmental degradation processes, and efficiency in reducing insects through its use. The H index for this dataset was 91. The cooperation network of the authors among countries showed the USA as the most notorious, with 30.6% of studies, followed by China (15.7%) and Brazil (10.9%). There are many studies on the toxicity of fipronil in bees, forms of degradation, and effectiveness of this insecticide. The present work presents suggestions pointed out in the articles for further research and highlights the importance of studies involving fipronil, as well as studies of alternative pest control.
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  • 文章类型: Journal Article
    Overuse of phosphorus (P) fertilizer and the resulting soil P accumulation in vegetable production increases the risk of P runoff and leaching. However, P transformations under continuous fertilization and their effects on environmental risk are unclear. The current study examined the effects of long-term P fertilizer application on P fractions in different soil layers, and assessed the correlations between P fractions and environmental risks in intensive vegetable production in a subtropical region. A total of 32 fields were studied, including 8 uncultivated fields and 24 fields continuously used for vegetable production for 1-3, 4-9, or 10-15 years. The results showed that excessive P fertilizer input caused soil P surpluses ranging from 204.6 to 252.4 kg ha-1 yr-1. Compared to uncultivated fields, vegetable fields contained higher levels of labile P, moderately labile P, sparingly labile P, and non-labile P. The combined percentage of labile P and moderately labile P increased from 55.2% in fields cultivated for 0-3 year to 65.5% in fields cultivated for 10-15 years. The concentrations of soil P fractions were higher at 0-20 cm soil depth than at 20-40 and 40-60 cm soil depth. Soil available P was positively correlated with all soil P fractions except diluted HCl-Pi or concentrated HCl-Po. Long-term vegetable production increased CaCl2-P downward movement, which was positively correlated with levels of labile and moderately labile P. The P index indicated a high risk of P losses from the vegetable fields. The P index was on average 3.27-fold higher in the vegetable fields than in uncultivated fields, and was significantly correlated with soil available P and organic and inorganic P fertilizer input. The environmental risk caused by P in vegetable production should be reduced by reducing P fertilizer input so as to maintain soil available P within an optimal range for vegetable production.
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  • 文章类型: Journal Article
    Uranium-enriched coal ash (CA) receives a significant attention as a supplementary nuclear resource also due to its potential environmental risk. Combining with CA, the changing trend of uranium occurrence in synthetic coal ash (SCA) was described at CaO-Al2O3-Fe2O3 ternary phase diagrams with a fixed SiO2 (wt. %, 30%, 50% and 70%) and Na2O (2%) content. This study reveals that the mode of uranium occurrence proposes a three-stage changing process during coal combustion including uranium oxidation, combination and encapsulation. Furthermore, a high frequency of encapsulated uranium resulted from the complicated interactions among major components with a medium SiO2 content, whereas the degree was higher at a higher SiO2, resulting in the decrease of uranium mobility. Uranium was encapsulated by Si-Al matrix and Fe-Si depletion if provided the high Al2O3 and Fe2O3 but low CaO contents. However, with the development of calcium looping and biomass co-firing process, the change of element mobility should be considered in industry owing to the extra-added alkaline metals. As the activation of Ca2+ induces a significant susceptibility of acid attack, cautions must be paid in CA with a higher Ca/Si ratio to avoid its utilization as constructive materials for the potential environmental risk.
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