pollution

污染
  • 文章类型: Journal Article
    微塑料(MPs),尺寸小于5毫米的微小塑料颗粒,已经成为海洋中常见而令人担忧的污染物,淡水,和世界各地的陆地环境。在这项研究中,我们揭示了Türkiye的两种特有new物种的微塑料暴露。我们发现,聚对苯二甲酸乙二醇酯(PET)是两种物种中主要的微塑料聚合物类型,特别是蓝色纤维的形状。我们还发现,微塑料大小与胃肠道(GIT)重量之间存在负相关,但是两种物种的体长和GIT重量之间没有显着差异。我们的发现可能会令人惊讶,因为所研究的物种生活在偏远的自然泉水中,高海拔地区。然而,在他们的栖息地发现水瓶似乎是他们暴露于微塑料污染的原因。因此,减少一次性塑料的使用预计将有助于保护这些特有的new。
    Microplastics (MPs), tiny plastic particles less than 5 mm in size, have emerged as a common and worrying pollutant in marine, freshwater, and terrestrial environments worldwide. In this study, we revealed the microplastic exposure of two endemic newt species for Türkiye. We found that polyethylene terephthalate (PET) was the predominant microplastic polymer type in both species, with the blue fiber shape in particular. We also found that there was a negative correlation between microplastic size and gastrointestinal tract (GIT) weight, but there was no significant difference between body length and GIT weight of both species. Our findings might be surprising as the studied species live in natural spring waters in remote, high-altitude areas. However, the detection of water bottles in their habitats appears to be the reason for their exposure to microplastic pollution. Therefore, reducing the use of single-use plastics is predicted to contribute to the conservation of these endemic newts.
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  • 文章类型: Journal Article
    由于生存的生态环境和人类生产活动不可避免地危及循环中药的安全性和治疗效果,因此循环中药中重金属的积累引起了广泛的关注。如何降低污染水平和改善毒性损害成为一个紧迫的问题。本文全面概述了重金属污染的现状,超过一千种单一草药(botanical,近二十年来出版的动物和矿物药物)和中药制剂。调查显示,生长生态系统(土壤,水源),人为因素(收获,processing,storage),利用的特定品种和药用部位以及固有的抗性能力是影响重金属在中药中积累的关键因素。Cu和Cr是植物药的主要累积元素,矿物和动物药物以As和Cu元素为主,分别。正在进行的努力旨在通过优化的培养过程来减轻重金属的水平和易位率,适当的处理方法和先进的吸附技术是有效的去除策略。并展望了TCMs作为重金属毒性损害的解毒剂的发展前景。此外,阐明砷(As)和铬(Cr)的形态与毒性之间的相关性,为规范药物剂量和周期提供有效参考。从提高动物药品HMs限制标准的角度来看,外用制剂和民间药物以及探索重金属与中药活性成分的相互作用机制为后续研究提供了方向。
    The accumulation of heavy metal in circulating TCMs has attracted widespread attention because the security and therapeutic efficacy are inevitably imperiled by the survival ecological environment and human production activities. How to reduce the pollution level and improve the toxicity damage becomes an urgent issue. This article provides a comprehensive overview of the current status of heavy metal contamination over a thousand types of single herbal (botanical, animal and mineral medicines) and TCM preparations published over nearly two decades. The survey revealed that growth ecosystems (soil, water sources), anthropogenic factors (harvesting, processing, storage), specific varieties and medicinal parts utilized as well as the inherent resistance capacity are the key factors that affect the accumulation of heavy metals in TCMs. And Pb, Cu and Cr are the major cumulative elements for botanicals, while mineral and animal medicines are dominated by As and Cu elements, respectively. Ongoing efforts aimed at mitigating the level and translocation rate of heavy metals by optimized cultivation processes, appropriate processing methodologies and advanced adsorption techniques are effective removal strategies. And the prospects of TCMs as a detoxifying agent for heavy metal toxicity damage posed development potential. Besides, the correlation between the speciation of arsenic (As) and chromium (Cr) and their toxicity should also be elaborated in order to provide effective references for standardizing drug dosage and cycle. And the imperative from the perspective of improving limitations standards of HMs for animal medicines, external preparations and folk medicines as well as exploring the interaction mechanisms between heavy metals and active ingredients of TCMs provides the direction for the follow-up study.
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  • 文章类型: Journal Article
    食物链中重金属和类金属(金属(类))的存在是一个全球性问题,因此,金属(类)被认为是潜在有毒元素(PTE)。砷(As),铅(Pb),汞(Hg),镉(Cd)被确定为与整个食物链中的人类健康风险相关的突出危害。这项研究旨在对北中部地区浅层表层土壤中的金属(类)进行来源归属,西北,和爱尔兰共和国的边境县,然后评估潜在的生态和人类健康风险。正矩阵分解(PMF)用于PTE的源表征,其次是蒙特卡罗模拟方法,用于评估潜在人类健康风险的概率模型。基于开源Tellus数据集,表层土壤中优先考虑的金属(类)的平均浓度范围为Pb(28.83mgkg-1)>As(7.81mgkg-1)>Cd(0.51mgkg-1)>Hg(0.11mgkg-1)。这项研究确定了金属(类)污染的三个主要来源:地质来源(36%),历史采矿和自然起源的混合来源(33%),和人为活动(31%)。生态风险评估表明,爱尔兰土壤呈现低-中度污染水平,对Cd和As水平的担忧仍然存在。除Cd外,所有金属(类)均显示出可接受的非致癌风险,而Cd和As占高到中等的潜在癌症风险。马铃薯消费量(如果在金属含量升高的土地上种植),土壤中Cd浓度,马铃薯中Cd的生物积累因子是最敏感的三个参数。总之,爱尔兰的金属(loid)存在低至中等的生态和人类健康风险。它强调需要制定政策和补救战略,以定期监测农业土壤中的金属(类)水平,并在金属(类)水平升高的地区生产生物累积性低的作物。
    The presence of heavy metals and metalloids (metal(loid)s) in the food chain is a global problem, and thus, metal(loid)s are considered to be Potentially Toxic Elements (PTEs). Arsenic (As), lead (Pb), mercury (Hg), and cadmium (Cd) are identified as prominent hazards related to human health risks throughout the food chain. This study aimed to carry out a source attribution for metal(loid)s in shallow topsoil of north-midlands, northwest, and border counties of the Republic of Ireland, followed by an assessment of the potential ecological and human health risks. The positive Matrix Factorization (PMF) was used for source characterization of PTEs, followed by the Monte Carlo simulation method, used for a probabilistic model to evaluate potential human health risks. The mean concentrations of prioritized metal(loid)s in the topsoil range in the order of Pb (28.83 mg kg-1) > As (7.81 mg kg-1) > Cd (0.51 mg kg-1) > Hg (0.11 mg kg-1) based on the open-source Tellus dataset. This research identified three primary sources of metal(loid) pollution: geogenic sources (36 %), mixed sources of historical mining and natural origin (33 %), and anthropogenic activities (31 %). The ecological risk assessment showed that Ireland\'s soil exhibits low-moderate pollution levels however, concerns remain for Cd and As levels. All metal(loid)s except Cd showed acceptable non-carcinogenic risk, while Cd and As accounted for high to moderate potential cancer risks. Potato consumption (if grown on land with elevated metal(loid) levels), Cd concentration in soil, and bioaccumulation factor of Cd in potatoes were the three most sensitive parameters. In conclusion, metal(loid)s in Ireland present low to moderate ecological and human health risks. It underscores the need for policies and remedial strategies to monitor metal(loid) levels in agricultural soil regularly and the production of crops with low bioaccumulation in regions with elevated metal(loid) levels.
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  • 文章类型: Journal Article
    本研究调查了1990年至2019年中国286个城市的开放度与污染物排放强度之间的关系,旨在评估开放型经济战略的潜在环境效益。研究结果表明,城市开放程度的提高显著降低了污染物排放强度。为了确保我们发现的稳健性,我们进行了创新尝试,将高铁连接和高速公路密度作为工具变量,以解决潜在的内生性问题,通过各种稳健性测试证实结果的可靠性。此外,我们还发现城市开放对污染排放的异质性影响,强调贸易复杂性的缓和影响,城市化水平,和环境监管强度。最后,这项研究阐明了城市开放减少污染排放的机制,即培养绿色创新能力和提高公众环境意识。这项研究为理解开放经济与环境保护之间的联系做出了理论贡献,同时为政府环境政策的制定提供了实用的见解。
    This study investigates the relationship between openness and pollutant emission intensity across 286 Chinese cities from 1990 to 2019, aiming to evaluate the potential environmental benefits of open economy strategies. The findings indicate that enhanced urban openness significantly lowers pollutant emission intensity. To ensure the robustness of our findings, we make an innovative attempt to employ high-speed rail connection and motorway density as instrumental variables to address potential endogeneity issues, corroborating the reliability of the results through various robustness tests. Moreover, we also find the heterogeneous effects of urban openness on pollution emissions, highlighting the moderating influences of trade complexity, urbanization level, and environmental regulatory intensity. Lastly, the study elucidates the mechanisms through which urban openness diminishes pollution emissions, namely fostering green innovation capacity and enhancing public environmental awareness. This research makes theoretical contributions on understanding the nexus between open economies and environmental protection while offering practical insights to inform governmental environmental policy formulation.
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  • 文章类型: Journal Article
    由于其技术和经济可行性,植物修复是一个快速扩展的过程。这项工作的目的是评估Helianthusannuus在三种培养基中的植物修复潜力:人工污染的加泰罗尼亚土壤,水培和路边土壤。在水培法中,使用ZnCl2剂量0.32mgL-1、29.94mgL-1、60.06mgL-1、119.94mgL-1。在人工污染的土壤中,剂量分别为0mgkg-1、299mgkg-1、599mgkg-1、1498mgkg-1。生理分析表明,处理T3和T4,金属的最高浓度,抑制生长并促进根部变黑。最高的Zn含量出现在地上部分。结果表明,Helianthusannuus由于其能够主要在人工污染的土壤中积累高水平的Zn而被归类为超积累。
    Phytoremediation is a rapidly expanding process due to its technical and economic viability. The objective of this work was to evaluate the phytoremediation potential of Helianthus annuus in three cultivation media: artificially contaminated Catalão soil, hydroponics and roadside soil. In hydroponics, ZnCl2 doses 0.32 mgL- 1, 29.94 mgL- 1, 60.06 mgL- 1, 119.94 mgL- 1 were used. While in the artificially contaminated soil, the doses were 0 mgkg- 1, 299 mgkg- 1, 599 mgkg- 1, 1498 mgkg- 1. Physiological analyzes made it possible to demonstrate that treatments T3 and T4, with the highest concentrations of the metal, inhibited growth and promoted darkening of the roots. The highest Zn contents occurred in the aerial part. The results indicated that Helianthus annuus was classified as hyperaccumulator due to its ability to accumulate high levels of Zn mainly in artificially contaminated soil.
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  • 文章类型: Journal Article
    巨藻氮同位素分析(δ15N)是鉴定氮污染物来源的可靠方法。了解小海湾和/或港口环境中的δ15N地理空间变化可以帮助确定氮污染的点源。这项研究对300多个岩藻和Ulvasp进行了采样。2022年9月和2023年5月来自Staites港的标本,北约克郡,英格兰。与Staites港和北海的站点相比,StaitesBeck的δ15N值升高:这归因于污水和/或农业粪便。Staites港内很少有站点在δ15N方面彼此显着不同,表明港口的氮同位素记录相对均匀。像Staites这样的简单港口环境可能相对较好地混合,因此,对一个港口地点进行采样可能足以代表整个港口。当然,更复杂的港口可能需要更多的样本位置来确定港口的点源和混合。
    Macroalgal nitrogen isotope analysis (δ15N) is a reliable method for the identification of nitrogen pollutant sources. Understanding δ15N geospatial variation within small bays and/or harbour environments can help identify point sources of nitrogen pollution. This study sampled over 300 Fucus vesiculosus and Ulva sp. specimens in September 2022 and May 2023 from Staithes Harbour, North Yorkshire, England. δ15N values for Staithes Beck were elevated when compared to sites in Staithes Harbour and the North Sea: this is attributed to sewage effluent and/or agricultural manure. Few sites within Staithes Harbour were significantly different from one another in terms of δ15N, suggesting a relatively homogenous nitrogen isotope record of the harbour. Simple harbour environments like Staithes may be relatively well mixed, and thus, sampling one harbour site may be enough to represent the entire harbour. Of course, more complex harbours may require more sample locations to ascertain point sources and mixing in the harbour.
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  • 文章类型: Journal Article
    新出现的证据表明,环境中的化学物质暴露是心血管疾病(CVD)的被忽视的驱动因素。最近的证据表明,主要来自塑料的化学或机械降解的微米和纳米塑料(MNP)颗粒可能代表了一种新的CVD风险因素。临床前模型中的实验数据表明,MNPs可以促进氧化应激,血小板聚集,细胞衰老,以及内皮细胞和免疫细胞的炎症反应,同时促进一系列可能导致疾病和过早死亡的心血管和代谢改变。在人类中,来自各种塑料的MNPs,包括聚乙烯和聚氯乙烯,已经在动脉粥样硬化斑块和其他心血管组织中检测到,包括心包,心外膜脂肪组织,心包脂肪组织,心肌炎,和左心耳.MNPs在血栓内具有可测量的水平,并且似乎优先在血管病变区域内积累。它们在颈动脉斑块内的存在与随后的心血管事件发生率增加有关。为了进一步研究MNPs在CVD中可能的因果作用,未来的研究应该集中在大,前瞻性队列评估个体暴露于塑料相关污染,可能的吸收途径,假定的安全限制的存在,组织中暴露和积累之间的对应关系,积累和CVD发展之间的时间,以及相关浓度的MNPs引起的病理生理机制。这些研究的数据将允许预防性设计,甚至是治疗,策略。同时,现有证据表明,减少塑料生产和使用将对环境和人类健康产生益处。这一目标可以通过目前正在谈判的《联合国全球塑料条约》来实现。
    Emerging evidence indicates that chemical exposures in the environment are overlooked drivers of cardiovascular diseases (CVD). Recent evidence suggests that micro- and nanoplastic (MNP) particles derived largely from the chemical or mechanical degradation of plastics might represent a novel CVD risk factor. Experimental data in preclinical models suggest that MNPs can foster oxidative stress, platelet aggregation, cell senescence, and inflammatory responses in endothelial and immune cells while promoting a range of cardiovascular and metabolic alterations that can lead to disease and premature death. In humans, MNPs derived from various plastics, including polyethylene and polyvinylchloride, have been detected in atherosclerotic plaques and other cardiovascular tissues, including pericardia, epicardial adipose tissues, pericardial adipose tissues, myocardia, and left atrial appendages. MNPs have measurable levels within thrombi and seem to accumulate preferentially within areas of vascular lesions. Their presence within carotid plaques is associated with subsequent increased incidence of cardiovascular events. To further investigate the possible causal role of MNPs in CVD, future studies should focus on large, prospective cohorts assessing the exposure of individuals to plastic-related pollution, the possible routes of absorption, the existence of a putative safety limit, the correspondence between exposure and accumulation in tissues, the timing between accumulation and CVD development, and the pathophysiological mechanisms instigated by pertinent concentrations of MNPs. Data from such studies would allow the design of preventive, or even therapeutic, strategies. Meanwhile, existing evidence suggests that reducing plastic production and use will produce benefits for the environment and for human health. This goal could be achieved through the UN Global Plastics Treaty that is currently in negotiation.
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  • 文章类型: Journal Article
    废机油是源自运输部门和工业重型机械操作的有害废油。处理不当,处置,和其他误用会导致大量空气,土壤,沉积物,地表水,和地下水污染。长期和反复接触的职业暴露会带来直接或间接的健康风险,导致短期(急性)或长期(慢性)毒性。土壤污染通过破坏土壤的生物群落和理化性质而引起地理毒性,和损害植物生长的植物毒性,生理和新陈代谢。地表水污染影响水生生态系统和生物多样性。焚烧造成的空气污染导致温室气体的释放,造成全球变暖,有害气体和颗粒物引起肺部疾病。废机油的毒性是由于总石油烃(TPH)成分,包括多环芳烃(PAHs),苯,甲苯,乙苯,二甲苯(BTEX),多氯联苯(PCBs)同源物,有机金属化合物,和有毒的化学添加剂。本文旨在全面概述生态毒理学效应,人类和动物健康毒理学和暴露于废机油。它突出了发动机油的特性和功能,并描述了废发动机油的产生,处置和回收。它提供了毒物动力学的深入评估和描述,新陈代谢,基于毒理学的人类和动物研究中的暴露途径和中毒,流行病学和实验研究。它强调了职业暴露的预防措施,并建议了基于风险的修复技术来减轻环境污染。审查将有助于了解废机油的潜在风险,同时考虑到公共卫生的益处和重要性。
    Waste engine oils are hazardous waste oils originating from the transportation sector and industrial heavy-duty machinery operations. Improper handling, disposal, and miscellaneous misuses cause significant air, soil, sediments, surface water, and groundwater pollution. Occupational exposure by prolonged and repeated contact poses direct or indirect health risks, resulting in short-term (acute) or long-term (chronic) toxicities. Soil pollution causes geotoxicity by disrupting the biocenosis and physicochemical properties of the soil, and phytotoxicity by impairing plant growth, physiology and metabolism. Surface water pollution impacts aquatic ecosystems and biodiversity. Air pollution from incineration causes the release of greenhouse gases creating global warming, noxious gases and particulate matter eliciting pulmonary disorders. The toxicity of waste engine oil is due to the total petroleum hydrocarbons (TPH) composition, including polycyclic aromatic hydrocarbons (PAHs), benzene, toluene, ethylbenzene, xylene (BTEX), polychlorinated biphenyls (PCBs) congeners, organometallic compounds, and toxic chemical additives. The paper aims to provide a comprehensive overview of the ecotoxicological effects, human and animal health toxicology and exposure to waste engine oils. It highlights the properties and functions of engine oil and describes waste engine oil generation, disposal and recycling. It provides intensive evaluations and descriptions of the toxicokinetics, metabolism, routes of exposure and toxicosis in human and animal studies based on toxicological, epidemiological and experimental studies. It emphasises the preventive measures in occupational exposure and recommends risk-based remediation techniques to mitigate environmental pollution. The review will assist in understanding the potential risks of waste engine oil with significant consideration of the public health benefits and importance.
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  • 文章类型: Journal Article
    目的:评估芝加哥城市家庭的家庭空气污染水平,并研究社会经济因素如何影响这些水平。方法:我们向芝加哥不同人口的244个家庭部署了无线空气监测设备,以连续记录家庭细颗粒物(PM2.5)浓度。我们计算了24小时周期内的每小时平均PM2.5浓度。四个因素-种族,家庭收入,面积剥夺,和吸烟暴露-在这项研究中被考虑。结果:共记录了93085小时的暴露数据。家庭PM2.5平均浓度为43.8μgm-3。我们观察到黑人/非裔美国人与非黑人/非裔美国人家庭之间的平均家庭PM2.5浓度存在显着差异(46.3对31.6μgm-3),在高收入和低收入家庭之间(18.2对52.5μgm-3),在吸烟和不吸烟家庭之间(69.7对29.0μgm-3)。然而,在较少和较少贫困地区的家庭之间没有观察到显著差异(43.7对43.0μgm-3).影响:芝加哥家庭的家庭空气污染水平远高于建议水平,挑战家庭空气质量适合高收入国家人口的假设。我们的结果表明,这是参与者的个人特征,而不是宏观环境,导致观察到的家庭空气污染差异。
    Purpose: To assess household air pollution levels in urban Chicago households and examine how socioeconomic factors influence these levels. Methods: We deployed wireless air monitoring devices to 244 households in a diverse population in Chicago to continuously record household fine particulate matter (PM2.5) concentration. We calculated hourly average PM2.5 concentration in a 24-hour cycle. Four factors-race, household income, area deprivation, and exposure to smoking-were considered in this study. Results: A total of 93085 h of exposure data were recorded. The average household PM2.5 concentration was 43.8 μg m-3. We observed a significant difference in the average household PM2.5 concentrations between Black/African American and non-Black/African American households (46.3 versus 31.6 μg m-3), between high-income and low-income households (18.2 versus 52.5 μg m-3), and between smoking and non-smoking households (69.7 versus 29.0 μg m-3). However, no significant difference was observed between households in less and more deprived areas (43.7 versus 43.0 μg m-3). Implications: Household air pollution levels in Chicago households are much higher than the recommended level, challenging the hypothesis that household air quality is adequate for populations in high income nations. Our results indicate that it is the personal characteristics of participants, rather than the macro environments, that lead to observed differences in household air pollution.
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