关键词: bioelectrodes biosensors enzymatic biofuel cells enzyme cascade implanted devices metal‐organic frameworks single enzyme biofuel cells

来  源:   DOI:10.1002/EXP.20220145   PDF(Pubmed)

Abstract:
The past few decades have seen increasingly rapid advances in the field of sustainable energy technologies. As a new bio- and eco-friendly energy source, enzymatic biofuel cells (EBFCs) have garnered significant research interest due to their capacity to power implantable bioelectronics, portable devices, and biosensors by utilizing biomass as fuel under mild circumstances. Nonetheless, numerous obstacles impeded the commercialization of EBFCs, including their relatively modest power output and poor long-term stability of enzymes. To depict the current progress of EBFC and address the challenges it faces, this review traces back the evolution of EBFC and focuses on contemporary advances such as newly emerged multi or single enzyme systems, various porous framework-enzyme composites techniques, and innovative applications. Besides emphasizing current achievements in this field, from our perspective part we also introduced novel electrode and cell design for highly effective EBFC fabrication. We believe this review will assist readers in comprehending the basic research and applications of EBFCs as well as potentially spark interdisciplinary collaboration for addressing the pressing issues in this field.
摘要:
在过去的几十年中,可持续能源技术领域的进步越来越快。作为一种新的生物和生态友好型能源,酶促生物燃料电池(EBFC)由于其可植入生物电子学的能力而获得了重要的研究兴趣,便携式设备,和生物传感器在温和的情况下利用生物质作为燃料。尽管如此,许多障碍阻碍了EBFC的商业化,包括它们相对适中的功率输出和酶的长期稳定性差。为了描述EBFC的当前进展并应对其面临的挑战,这篇综述追溯了EBFC的演变,并聚焦于当代的进展,如新出现的多酶系统或单酶系统,各种多孔框架-酶复合材料技术,创新应用。除了强调这一领域目前的成就外,从我们的角度来看,我们还介绍了用于高效EBFC制造的新型电极和电池设计。我们相信这篇评论将帮助读者理解EBFC的基础研究和应用,并可能引发跨学科合作,以解决该领域的紧迫问题。
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